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Electoral lists of the commotes of: Ardudwy Uwch Artro, 1860-1861; Ardudwy Is Artro, 1861; Mawddwy, [1860s]; Tal-y-bont, 1861-1863; and Ystumanner, 1860; and jury lists for the parishes of Beddgelert; Dolgellau; Llanfihangel-y-Pennant; Llanfihangel-y-traethau; Llanfrothen; Llangelynnin; and Trawsfynydd, 1866.

Records and papers collected by Emrys Roberts, 1945-1983, including correspondence and papers relating to the National Eisteddfod, 1959-1976; the Development Board for Rural Wales, 1973-1981; and Wales (West and North) Television Ltd, 1960-1967. There are also papers relating to other committees on which Emrys Roberts sat, 1967-1983, and other miscellaneous papers, 1945-1981.

Press letter books, 1878-1920, press invoice books, 1878-1919, account books, 1893-1920, and a minute book, 1900-1901.

Deeds and documents of the Bennett family of Glanyrafon, Montgomeryshire, and the Owen family of Dolgoed and Llawrpenegoes, 1546-1946, relating mainly to properties in the parishes of Llanidloes, Llanwrin, Penegoes, and Trefeglwys, Montgomeryshire, and Talyllyn, Merionethshire; and a map of properties in Trefeglwys, 1819.

Papers of Elizabeth Baker, 1740-1798, comprising correspondence, 1743-1798; copies of verses, including some relating to the impeachment of Warren Hastings; correspondence relating to legal matters arising from the mining partnership and the ownership of the Nannau estate, 1779-1781; journals relating to silk worms, 1779-1782; and papers concerning politics, literature, and current events, 1740-1798.

Deeds, 1555-1918, of clients and relating to properties in Cardiganshire, Merionethshire, Montgomeryshire and Radnorshire, including papers of the Penglais estate in the Aberystwyth area, 1555-1918; Aberystwyth borough records, 1759-1813; letters, 1794-1882; papers of John Parry, solicitors, Aberystwyth, including share certificates of the Aberystwyth Gas and Coke Company, 1839; Bwlch Consolidated Lead Mines, 1847; records concerning the Aberystwyth and Tregaron Bank, 1813-1844; miscellaneous papers, [c. 1783]-1932; printed items, [c. 1783]-1867; certificates of shares in the Aberystwyth Public Rooms, 1818-1821, and the Robinson Gold Mining Company, 1903; letters and papers relating to the estate of Roderick Richards, Penglais, [c. 1830]; builders' accounts, 1845; and tithe receipts, 1927-1932.

Deeds, documents and plans, 1455-1895, relating to properties in Anglesey, Caernarfonshire, Denbighshire, Merionethshire and Montgomeryshire; including papers of the Poole family, owners of the Caenest and Pencraig estates in Merionethshire and Anglesey; surveys, [c. 1770] of the Caenest and Pencraig estates; and building leases for properties in the port of Amlwch, [late 18th century].