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Papers of the Pale estate belonging to Henry Beyer Robertson, 1879-1950, comprising correspondence on Council matters, especially the contract between Bala Urban District Council and Merionethshire County Council for the upkeep of the main roads, 1880-1948; pamphlets, diagrams and letters concerning the Pale hydro-electric plant, 1892-1936; and miscellaneous papers, 1885-1948, including items relating to the 1885 general election campaign in Merionethshire.

Deeds and documents, 1598-1856, mostly assignments of mortgage and related bonds, concerning Dôl y Cae and other premises in the parish of Tal-y-llyn, including a lease from William Owen Pughe and his brother Richard to his son Aneurin Owen Pughe.

Electoral lists of the commotes of: Ardudwy Uwch Artro, 1860-1861; Ardudwy Is Artro, 1861; Mawddwy, [1860s]; Tal-y-bont, 1861-1863; and Ystumanner, 1860; and jury lists for the parishes of Beddgelert; Dolgellau; Llanfihangel-y-Pennant; Llanfihangel-y-traethau; Llanfrothen; Llangelynnin; and Trawsfynydd, 1866.

Records and papers collected by Emrys Roberts, 1945-1983, including correspondence and papers relating to the National Eisteddfod, 1959-1976; the Development Board for Rural Wales, 1973-1981; and Wales (West and North) Television Ltd, 1960-1967. There are also papers relating to other committees on which Emrys Roberts sat, 1967-1983, and other miscellaneous papers, 1945-1981.

Press letter books, 1878-1920, press invoice books, 1878-1919, account books, 1893-1920, and a minute book, 1900-1901.

Deeds and documents of the Bennett family of Glanyrafon, Montgomeryshire, and the Owen family of Dolgoed and Llawrpenegoes, 1546-1946, relating mainly to properties in the parishes of Llanidloes, Llanwrin, Penegoes, and Trefeglwys, Montgomeryshire, and Talyllyn, Merionethshire; and a map of properties in Trefeglwys, 1819.

Papers of Elizabeth Baker, 1740-1798, comprising correspondence, 1743-1798; copies of verses, including some relating to the impeachment of Warren Hastings; correspondence relating to legal matters arising from the mining partnership and the ownership of the Nannau estate, 1779-1781; journals relating to silk worms, 1779-1782; and papers concerning politics, literature, and current events, 1740-1798.

Deeds, 1555-1918, of clients and relating to properties in Cardiganshire, Merionethshire, Montgomeryshire and Radnorshire, including papers of the Penglais estate in the Aberystwyth area, 1555-1918; Aberystwyth borough records, 1759-1813; letters, 1794-1882; papers of John Parry, solicitors, Aberystwyth, including share certificates of the Aberystwyth Gas and Coke Company, 1839; Bwlch Consolidated Lead Mines, 1847; records concerning the Aberystwyth and Tregaron Bank, 1813-1844; miscellaneous papers, [c. 1783]-1932; printed items, [c. 1783]-1867; certificates of shares in the Aberystwyth Public Rooms, 1818-1821, and the Robinson Gold Mining Company, 1903; letters and papers relating to the estate of Roderick Richards, Penglais, [c. 1830]; builders' accounts, 1845; and tithe receipts, 1927-1932.

Deeds, documents and plans, 1455-1895, relating to properties in Anglesey, Caernarfonshire, Denbighshire, Merionethshire and Montgomeryshire; including papers of the Poole family, owners of the Caenest and Pencraig estates in Merionethshire and Anglesey; surveys, [c. 1770] of the Caenest and Pencraig estates; and building leases for properties in the port of Amlwch, [late 18th century].

Papurau Bob Owen yn cynnwys traethodau eisteddfodol, 1910-1941; beirniadaethau ar draethodau eisteddfodol, 1916-1949; crynodebau o bregethau a glywodd, 1895-1927; teipysgrifau rhaglenni radio yr oedd ynghlwm wrthynt, 1936-1957; gohebiaeth, 1908-1961, yn cynnwys llythyrau Dr Thomas Richards, 1923-1960; dyddiaduron, 1905-1961; papurau personol, 1898-1961; papurau teuluol, 1900-1923; copïau a drafftiau o ddarlithoedd, erthyglau a thraethodau, 1906-1950; nodiadau ac adysgrifau helaeth ganddo o farddoniaeth Gymraeg, ewyllysiau a mynegeion ewyllysiau, cartiau achau ac achresi, cofrestri plwyf ac adysgrifau'r esgob, dyddiaduron, llythyrau, almanaciau, cofnodion llys, yn ymwneud yn bennaf â siroedd Caernarfon a Meirionnydd, a chofiannau, [20 gan., ½ cyntaf]; nodiadau ar anghydffurfiaeth yng Ngogledd Cymru, plwyfi siroedd Meirionnydd a Chaernarfon, llongau a morwyr o Gymru a Chymry Llundain, [20 gan., ½ cyntaf]; nodiadau pwysig ar ymfudo o Gymru, yn enwedig i'r Unol Daleithiau, [20 gan., ½ cyntaf]; copïau teipysgrif o gofnodion corfforaethau yn cynnwys Parc Cenedlaethol Eryri a Chyngor Sir Feirionnydd, 1922-1962; cofnodion gwreiddiol a ddaeth i feddiant Bob Owen, yn bennaf cofnodion Chwarel Parc a Chroesor, sir Feirionnydd, yn cynnwys cyfrifon a chofnodion, 1891-1941, a chofnodion ysgolion ac ysgolion Sul, 1861-1957; a thorion ac adysgrifau o amrywiol gyfnodolion Cymreig, 1816-1965. = Papers of Bob Owen including eisteddfod essays, 1910-1941; adjudications of eisteddfod essays, 1916-1949; summaries of sermons heard by him, 1895-1927; typescripts of radio programmes involving him, 1936-1957; correspondence, 1908-1961, including letters from Dr Thomas Richards, 1923-1960; diaries, 1905-1961; personal papers, 1898-1961; family papers, 1900-1923; copies and drafts of lectures, articles and monographs, 1906-1950; extensive notes and transcripts by Bob Owen of Welsh poetry, wills and indexes of wills, pedigrees and genealogies, parish registers and bishops' transcripts, diaries, letters, almanacs, court records, mainly relating to Caernarfonshire and Merionethshire, and biographies, [20 cent, first ½]; notes on nonconformists in North Wales, Merionethshire and Caernarvonshire parishes, Welsh ships and sailors and the London Welsh, [20 cent, first ½]; important notes on emigration from Wales, especially to the United States, [20 cent, first ½]; typescript records of bodies including Snowdonia National Park and Merioneth County Council, 1922-1962; original records acquired by Bob Owen, mainly records of Parc and Croesor Quarry, Merionethshire, including accounts and minutes, 1891-1941, and school and Sunday School records, 1861-1957; and cuttings and transcripts from various Welsh periodicals, 1816-1965.