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Literary papers, 1964-1995, juvenilia, 1939-1942, and journals, 1966-1994, of Alison Bielski, together with her work journals, 1995-2002 .

A large collection of Alistair Crawford's papers relating to his academic and artistic career in Wales.

Deeds, mainly relating to the Alltlwyd estate, 1617-1869, chiefly in the parishes of Llanrhystud and Llansanffraid, Cardiganshire.

Papers of Alun Lewis, 1919-1996, including family correspondence and letters from Robert Graves; autograph and typescript copies of published and unpublished poems; typescript copies of published and unpublished prose; personalia; an unpublished autobiographical novella of college life; memorial tributes to Alun Lewis in poetry form; and notebooks containing poetry and other writings by him.

Papers of Alun-Oldfield Davies, 1928-1988, relating mainly to the artist and writer David Jones, including an original water-colour inscription, 1954; photographs of inscriptions, personalised and sent as greetings cards , 1958-1961; letters from David Jones to Alun Oldfield-Davies, 1954-1962; papers concerning the fate of David Jones's manuscripts and pictures, 1971-1976; miscellaneous items including lists of works by David Jones for exhibitions, 1972-1976, a radio talk broadcast in 1954 and articles on his life and work, 1954-1988. The additional papers comprise a copy of John Morris-Jones, Penillion Omar Khayyam (Gregynog Press, 1928), formerly in the possession of Colonel Richard C. Ruck (1887-1973), containing his manuscript annotations in Persian, Welsh and English, with letters from his widow concerning the bequest of the volume to Alun Oldfield-Davies, 1973-1974; and a notebook containing reminiscences in Welsh ('Stori fy mywyd') of the Reverend Jonathan Oldfield-Davies (1876-1960), Congregationalist minister and father of Alun Oldfield-Davies.

Personal papers of the photographer Alvin Langdon Coburn consisting mainly of correspondence concerning his association with several orders of freemasonry, 1903-1966. There is also a small amount of correspondence relating to his work as a photographer, 1913-1965, mainly concerning lectures broadcast by the BBC, but also including letters relating to the sale, by Coburn, of a small collection of letters from the American writer Henry James. The fonds also consists of lectures and associated notes, again mainly concerning Coburn's interest in freemasonry, 1937-[1966], dealing particularly with its history and origins; a few lectures reflecting particular aspects of his career as a photographer, and on his approach to photography, 1924-[1966]; together with some printed material, 1924-1966, primarily circulars from various Masonic lodges concerning forthcoming events. Given Coburn's important contributions to photography there is surprisingly little material which is of direct relevance to this aspect of his life within the archive. The additional group of material consists mainly of correspondence and papers relating to the administration of the estate of Alvin Langdon Coburn following his death and includes copies of his will and codicil and a Probate document proved at Bangor.

Papers, 1966-2015, relating to the filming and production of Under Milk Wood (1972), directed by Andrew Sinclair, together with papers relating to the financing and distribution of the film and to other Dylan Thomas projects.

Deeds, 1704-1912, relating to properties in the town of Denbigh and the parishes of Henllan and Eglwys-bach, Denbighshire.

Deeds, 1490-1977, including deeds and documents mainly relating to properties on Anglesey, Caernarfonshire, Merionethshire and Middlesex, 1675-1977; and deeds relating to properties in Finchley, Middlesex, 1490-1796.

Records relating to the Anglo-Welsh Review, mainly typescripts of material published in the magazine, 1957-1988, including editor's correspondence files, printer's copies and galley proofs, 1957-1988; and subscription lists, 1957-1975. The archive also includes correspondence and papers relating to the publication's demise and closure, 1981-2000 (November 2021 deposit).

A visitors book and two 'rotation books' (session lists) relating to the studio of the photographer Angus McBean, 1945-1987.

Sub-fond A comprises papers related to Ann Jones's campaign for domestic fire safety measures in Wales, centering on the devolution of powers to the National Assembly for Wales for this purpose and the resulting legislation; the Domestic Fire Safety (Wales) Measure, 2011, which required sprinkler systems to be fitted to all newly built or substantially converted domestic residences in Wales. Sub-fond B comprises material related to Ann Jones' campaign against the closure of the North Wales Fire and Rescue Service control room in Rhyl. Sub-fonds C comprises material related to the Children's Society's decision to withdraw from Wales, and Ann Jones' efforts in the the subsequent establishment of Tros Gynnal Plant to continue that work. Sub-fonds D relates to the restructure of the National Health Service in Wales.

Personal archive of material relating to Gwasg Gregynog accumulated by the donor during his time as a director and trustee of the Press, 1998-2018.

The archive includes papers and letters of members of the Anwyl family of Chester, 1848-1983, including letters to Sir Edward Anwyl, Welsh scholar.

This collection comprises notebooks containing poetry, sermons, etc. by Robert Thomas (Ap Vychan) (1809-1880), Congregational minister, poet, etc.

A collection comprising documents relating to the families of George Wade Green of Court Henry, Richard Thomas Howell of Bryncaerau, Francis Green of Denmark Hill, and Peter Williams of Gelli Lednais; also material relating to Cadwallader Jones, Collector General of the Customs to Charles I.

The collection known as the Archdeacon A. O. Evans Manuscripts is a group of manuscripts given to the National Library by Albert Owen Evans. They include correspondence and papers relating to A. O. Evans.

Papurau, 1974-1995 (1981-1994 yn bennaf), yn cynnwys sgriptiau, manylion parthed gwahanol weithdai a chynyrchiadau (gan gynnwys rhai gan gwmnïau eraill), papurau gweinyddol a chyllidol, cofnodion a gohebiaeth pwyllgorau, a phapurau yn ymwneud â pherfformwyr, theatrau a sefydliadau theatrig eraill yng Nghymru (yn cynnwys Cymdeithas Theatr Cymru, 1975-1990, Theatr Gymraeg Gwynedd, 1985-1988, Cymdeithas Ddrama Cymru, 1991-1992, a Chymdeithas Celfyddydau Perfformiadol Cymru, 1983-1994), ynghyd â lluniau, posteri a rhaglenni = Papers, 1974-1995 (mainly 1981-1994), comprising scripts, details regarding various workshops and productions (including some by other companies), administrative and financial papers, committee minutes and correspondence, and papers relating to performers, theatres and other Welsh theatrical organizations (including Cymdeithas Theatr Cymru, 1975-1990, Theatr Gymraeg Gwynedd, 1985-1988, Cymdeithas Ddrama Cymru, 1991-1992, and the Society of Performing Arts in Wales, 1983-1994), together with photographs, posters and programmes.

Papurau, 1972-1979, Cell Casnewydd o Gymdeithas yr Iaith Gymraeg, yn cynnwys gohebiaeth yn ymwneud â statws yr iaith mewn addysg, busnes a bywyd cyhoeddus yng Ngwent. = Papers, 1972-1979, of Cell Casnewydd, Cymdeithas yr Iaith Gymraeg, including correspondence relating to the status of the language in education, business and public life in Gwent.

Mae'r archif yn cynnwys: pamffledi, cylchlythyron etc., amrywiol; dwy gyfrol o gofnodion cyfarfodydd Pwyllgor Canolog (1967-70) a Senedd (1970-Ionawr 1975) Cymdeithas yr Iaith Gymraeg a rhai y cyfarfodydd cyffredinol blynyddol; cofnodion y Senedd,1974-1981 ac adroddiadau gan wahanol grwpiau o'r Gymdeithas, 1976-1981; papurau gweinyddol,1970-1981, yn cynnwys copïau o benderfyniadau a gyflwynwyd yng nghyfarfodydd cyffredinol y Gymdeithas a deunydd printiedig; papurau yn ymwneud â Grŵp y Dysgwyr, 1974-1985; papurau yn ymwneud â Mudiad Rhyddid yr Iaith, 1977; papurau yn ymwneud ag ymgyrchoedd y bu'r Gymdeithas yn eu canlyn,1970-1981, gan gynnwys yr ymgyrch dros sianel deledu Cymraeg; ffeiliau gohebiaeth,1966-1986; ffeiliau swyddfa,1971-1981; datganiadau i'r wasg etc., 1970-1990; cofnodion y Senedd,1979-1991; ffeiliau amrwiol,1975-1991; papurau yn ymwneud â darlledu, 1974-1980; ffurflenni aelodaeth, 1979-1990; papurau ynghylch y grŵp addysg, 1982-1989; papurau ynghylch tanysgrifiadau i Tafod y Ddraig, 1980-1990; llyfrau lloffion, 1965-1967, yn cynnwys papurau yn adlewyrchu ymgyrchoedd a gweithgareddau y Gymdeithas; cofnodion cyfarfodydd, 1966; atgofion am sefydlu'r Gymdeithas yn 1962 a'i datblygiad cynnar; amrywiol dorion o'r wasg; a phosteri amryfal. Y mae grŵp Mai 1996 yn cynnwys papurau, 1971-1993, yn ymwneud â gwahanol ranbarthau y Gymdeithas a phapurau,1984-1993, yn ymwneud â'i chynghorau, cyfarfodydd seneddol etc. Y mae'r grŵp mawr o gofnodion a dderbyniwyd ym mis Gorffennaf 1998 a mis Ionawr 1999 yn cynnwys y canlynol: llyfrau lloffion,1971-1996,yn cynnwys torion o'r wasg yn disgrifio ymgyrchoedd a gweithgareddau y Gymdeithas a bywyd gwleidyddol Cymru; papurau yn ymwneud ag Eisteddfod Genedlaethol yr Urdd a'r Eisteddfod Genedlaethol, 1986-1994, gohebiaeth oddi wrth y Swyddfa Ganolog,1988-1997; papurau ynglŷn â chelloedd a rhanbarthau y Gymdeithas, 1977-1996; papurau gweinyddol, 1977-1998, yn cynnwys dyddiaduron swyddfa, rhestrau aelodaeth, papurau yn perthyn i wahanol swyddogion y Gymdeithas, papurau ynglŷn â grŵp addysg y Gymdeithas, deunydd yn deillio o lawer o ymgyrchoedd y Gymdeithas, papurau ynglŷn â chyrsiau ar gyfer dysgwyr, papurau ynglŷn â'r Ddeddf Eiddo, a datganiadau i'r wasg. = The archive comprises: a series of forms bearing signatures supporting the Welsh Language Society's Petition to the new local authority bodies in Wales requesting them to strengthen the Welsh Language and Welsh Society; a series of forms bearing signatures supporting the Society's declaration of support for the workers of Shotton; miscellaneous pamphlets, circulars; etc.; two volumes of minutes of meetings of the Central Committee (1967-70) and Senate (1970-January 1975) of the Welsh Language Society and of some of the annual general meetings; minutes of the Senate, 1974-1981 and reports from various groups of the Society, 1976-1981; administrative papers, 1970-1981, including copies of resolutions presented to the general meetings of the Society and printed matter; papers concerning the Learners' Group, 1974-1985; papers concerning the Language Freedom Movement, 1977; papers concerning the campaigns pursued by the Society, 1970-1981, including the campaign for a Welsh language television channel; correspondence files, 1966-1986; office files, 1971-1981; press releases etc., 1970-1990; Senate minutes, 1979-1991; miscellaneous files, 1975-1991; papers relating to broadcasting, 1974-1980; membership forms, 1979-1990; papers concerning the education group, 1982-1989; papers concerning subscriptions to Tafod y Ddraig, 1980-1990; scrapbooks, 1965-1967, containing papers reflecting the campaigns and activities of the Society; minutes of meetings, 1966; reminiscences on the establishment of the Society in 1962 and its early development; miscellaneous press cuttings; and miscellaneous posters. The May 1996 group comprises papers, 1971-1993, relating to the various regions of the Society and papers, 1984-1993, relating to its councils, parliamentary meetings etc. The large group of records received in July 1998 and January 1999 comprise the following: scrapbooks, 1971-1996, containing press cuttings describing the campaigns and activities of the Society and Welsh political life; papers relating to the Urdd National Eisteddfod and the Welsh National Eisteddfod, 1986-1994, correspondence from the Central Office, 1988-1997; papers concerning cells and regions of the Society, 1977-1996; administrative papers, 1977-1998, including office diaries, membership lists, papers belonging to various officials of the Society, papers concerning the Society's education group, material deriving from many of the Society's campaigns, papers concerning courses for Welsh learners, papers concerning the Property Act, and press releases.