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Mae'r casgliad yn cynnwys papurau teuluol a phersonol,1913-1997, gan gynnwys tystysgrifau cofrestru sifil, gohebiaeth deuluol, tystysgrifau'n ymwneud â chysylltiad Huw Tudor â'r Seiri Rhyddion, a thaflenni gwasanaethau angladdau; papurau yn ymwneud â'r theatr, 1953-1993, yn cynnwys deunydd yn ymwneud â chyfnod Huw Tudor yn RADA, rhaglenni theatr a thorion perthynol o'r wasg; a phapurau amrywiol, 1957-1998, yn cynnwys torion o'r wasg ynglŷn â rhannau Huw Tudor ar y radio a'r teledu, deunydd yn ymwneud â'r Teulu Brenhinol, taflenni gwasanaethau coffa, a thestunau erthyglau a ysgrifennwyd gan Huw Tudor. = The collection comprises family and personal papers, 1913-1997, including civil registration certificates, family correspondence, Huw Tudor's freemasonry certificates, and funeral service cards; papers concerning the theatre, 1953-1993, including material concerning Huw Tudor's period at RADA, theatre programmes and related press cuttings; and miscellaneous papers, 1957-1998, including press cuttings concerning Huw Tudor's radio and television roles, material relating to the British Royal Family, memorial service cards, and the texts of articles written by Huw Tudor.

The collection comprises: Group 1: papers, 1997-1998, deriving from the Cardiff HQ of the 'Yes for Wales' campaign, including correspondence, strategy papers, minutes of committees and sub-groups, campaign materials, conference papers, financial papers, material emanating from the various Yes Supporting Groups, and papers deriving from several local support groups, among them Swansea, Pontypridd, Ceredigion and Neath. Group 2 consists of correspondence, press releases, governmental publications, strategy papers and campaign materials, 1997-1998. Group 3 comprises correspondence, minutes and agenda, strategy papers, financial papers, membership papers, press and media papers, newsletters, volumes of press cuttings, papers relating to each of the political parties in Wales, other support groups and a few papers relating to the 'No' campaign in 1997.

General personal and political correspondence, 1936-1997, including letters from the Royal Family, MPs and Government Ministers, such as James Callaghan, Margaret Thatcher and John Major; subject files including the Labour Party, 1951-1979, the National Union of Teachers, 1963-1971, Secretary of State for Wales, 1968-1969, Devolution in Wales, 1970-1973, the Christian Heritage, 1977-1985, Aberfan Disaster Fund Bill, 1978-1979, Cardiff West Constituency Labour Party, 1981-1982, the National Children's Homes, 1981-1993, British housing, 1984-1985, GT's memoirs, 1983-1985, the College of Preceptors, 1982-1987, the House of Lords, 1985-1987, St George's House, Windsor Castle, 1985-1987, education, 1986-1987, European Union, 1990-1997, the Welsh Assembly, 1996-1997, the WDA, 1991-1992, and various medical and charitable foundations, 1982-1997; miscellaneous political and personal papers, 1927-1997, including material concerning the Cardiff City Labour Group; 1927-1958; religious interests, 1960's-1990's; Speaker's engagements and official papers, 1976-1983; general publications, 1950-1987, including The Gospel Witness, 1955-1983; Parliamentary publications, 1961-1986, The House Magazine, 1980-1991; personal papers, [c. 1940s]-[1990s]; political papers, accumulated as MP for Cardiff West, Government Minister and Member of the House of Lords, 1955-1997; and letters, 1983-1997, from Sir Julian Hodge, relating to European union and devolution.

Papers of Elvey MacDonald, Patagonia, 1985-1997, mainly relating to the establishment of the Welsh radio programme Radio Ceredigion, Cardiganshire, 1985-1997; they include papers relating to various committees, 1985-1995, correspondence, 1985-1996; newspaper cuttings, 1985-1993.

Papers of Stuart Rendel and family members, including papers relating to the University College of Wales, Aberystwyth, and the proposal to establish the National Library of Wales and its development during the early years of its existence, 1883-1916; speeches, addresses and political papers relating to disestablishment of the church in Wales and the 1889 Intermediate Education Act, 1882-1909; press cuttings, 1881-1913; photographs, 1892; miscellaneous letters, 1878-1912; letters to Stuart Rendel, 1853-1912, including letters from A. C. Humphreys Owen, 1877-1905, family letters, 1853-1902, and letters from prominent political figures and Welsh public figures; letters and copies of letters from Rendel, 1880-1912; diaries, mainly recording details of Stuart Rendel's business activities, 1863-1869; notes of conversations with W. E. Gladstone, John Morley and H. H. Asquith, 1888-1910; papers relating to Chinese affairs and French and Chinese peace talks, 1884-1886; papers of James Meadows Rendel, including letters, 1828-1856, and papers relating to his estate, 1856-1859; letters of Catherine Jane Rendel, 1845-1855; letters and papers of George Wightwick Rendel, 1871-1902; papers relating to Rendel's other brothers, 1841-1889, and his daughters, 1882-1910; letters and papers of Harry Stuart Goodhart-Rendel, 1898-1959, and other papers concerning him, 1963-1977; papers, mainly letters, of the Goodhart family, 1819-1957; papers of Miss Rosemary Rendel, 1986-1996; papers of Sir George William Rendel, including: Foreign Office papers, 1917-1967, correspondence, 1912-1973, papers relating to the Catholic Union of Great Britain, 1942-1979, lectures, diaries and notes, 1915-1954, personal and family papers, 1908-1980, and material relating to the book The Sword and the Olive (1957), 1954-1986.

Papers, 1883-1996, of, or acquired by, the artist Ray Howard-Jones (1903-1996), including correspondence, diaries, notes and draft poems, and papers relating to exhibitions, together with photographs and slides, and printed material.

A further group of papers of, or acquired by Ray Howard-jones was received June 2006. This group remains uncatalogued.

Papers of Alun Lewis, 1919-1996, including family correspondence and letters from Robert Graves; autograph and typescript copies of published and unpublished poems; typescript copies of published and unpublished prose; personalia; an unpublished autobiographical novella of college life; memorial tributes to Alun Lewis in poetry form; and notebooks containing poetry and other writings by him.

The fonds comprises two accruals containing papers, 1985-1996, accumulated by Mike Webb and include papers relating to the Nicaraguan election of 1990; various environmental projects in Nicaragua, especially in the Ocotal region, 1986-1992; newspaper cuttings from Nicaragua and Britain, 1988-1994; newsletters, articles and posters relating to Central America, 1985-1993; papers reflecting the activities of the Grŵp Canolbarth America Môn Arfon Central America Group and other related organisations, 1987-1996; and papers concerning the Tom Hargreaves Memorial Fund, 1987-1995.

Cofysgrifau Capel Trinity, Llanelli gan gynnwys llyfr cofnodion cyfarfod Blaenoriaid, 1979-2008; cofnodion, 1892-1906, 1907-1928, 1922-1930 a 1938-1987; deg cyfrol yn perthyn i'r Ysgol Sul, 1909-1939, 1931-?, 1938-1946, 1940-1950, 1946-1950, 1951-1956, 1951-1956, 1956-1963, 1964-1975 a 1975-1995; ffolder drama Evan Roberts; ewyllys Mrs Elizabeth Ann Joel; adroddiadau Trinity; llyfryn hanes Trinity; a phapurau amrywiol eraill.

Development Board for Rural Wales records, containing minutes and other papers of the Board and various committees, 1977-1994; general administrative files concerning the establishment of the Board, its functions and responsibilities, and correspondence with other organizations, 1966-1990; construction files containing correspondence, contracts and estate plans relating to housing and industrial developments executed by the Board, particularly in Newtown, 1968-1993; records such as correspondence, minutes, notes and other papers relating to research studies on economic and social life in Mid-Wales carried out by the Board, 1968-1995; files relating to the Board's marketing and promotional strategy, 1978-1991; and press releases, 1977-1990; Mid-Wales Development Corporation records, 1962-1979, including annual reports, 1969-1977, minutes and papers of the Board and various committees, 1968-1979, and seal registers relating to MWDC projects, 1968-1976, containing compulsory purchase orders, contracts, leases and other documents.

An additional three files relating to the Development Board for Rural Wales, being DB/CF/101/1; DB/CF/101/2; DB/CF/101/3 – (Extension to Goodall & Swanwick factories at Dolgellau; factories at Dolgellau; and extension to Marian Park Industrial Estate, Dolgellau). These remain uncatalogued, and are closed for ten years from the date of the latest document in each file.

The music manuscripts of the composer David Harries, 1952-1995, comprising mainly drafts and scores of chamber and instrumental music, orchestral music, choral and organ, and voice and piano arrangements.
A second donation made in August 2021 contains further music manuscripts of David Harries, 1953-1993, and includes works by Harries' contemporary William Mathias (1934-1992) in addition to Harries' own compositions of chamber and instrumental music, orchestral music, choral and organ, and voice and piano arrangements.

Material largely relating to scripts and screenplays submitted to Ffilm Cymru; together with further Ffilm Cymru material, which includes proposals for film/television adaptations, casting and funding applications, employment enquiries, contracts and agreements, accounts and invoices, card indexes and correspondence.

The fonds comprises the literary and personal papers of Glyn Jones, 1814-1995 (with gaps), including manuscript and typescript drafts of poetry and prose works by him, related correspondence and press cuttings, radio scripts, talks and readings and adjudications. Also included are notes and articles pertaining to Glyn Jones, general correspondence and notebooks; various papers relating to members of his family; and works by other writers.

Papers relating to fringe Nationalist and left wing groups, 1963-1989, including material relating to Welsh Nationalist and Republican Groups, 1963-1989, material relating to Welsh left wing groups, 1969-1979, and papers relating to solidarity groups and campaigns, 1968-1989; published political material such as newspapers and periodicals, 1913-1989, records and papers of Cofiwn, 1970-1990, including material relating to the American Indian Movement Tour of Wales, 1986; papers relating to campaigns and activities of groups such as the the Owain Glyndwr Society, 1975-1990; papers relating to maritime history and heritage, 1973-1995; and miscellaneous papers, mainly relating to organisations in Aberystwyth, 1976-1989.

Papers, 1897-1994, of Geraint Dyfnallt Owen mainly comprising correspondence and travel journals reflecting Owen's involvement with Welsh and European history, politics and culture. There are also letters, 1929-1951, to and from Owen and his parents the Rev. and Mrs John Dyfnallt Owen. Letters from Breton cultural and religious leader Jean-Marie (Yann-Vari) Perrot, donated with other papers by Dr Geraint Dyfnallt Owen in 1979, have been incorporated in this group (NLW MS 23322D).

Papers, 1743-1994, of or relating to Margaret Mostyn Jones of Wern House, Mostyn, Flintshire, and to members of her family, and including a journal, 1861-1864, kept by her while employed by Augusta Hall, Lady Llanover; correspondence, 1876-1932, to and from Margaret Mostyn Jones, including letters, 1890-1894, written to members of her family while living in Ohio; an autobiographical essay, 1929-1932, by Margaret Mostyn Jones; together with papers, 1743-1874, mainly of Flintshire interest.

Papers, 1966-1994, comprising letters and cards to the playwright Dedwydd Jones, mostly from actors, playwrights and other prominent theatrical and literary figures.

Papurau Gwenlyn Parry, [1962]-1993, yn cynnwys sgriptiau a phapurau amrywiol yn ymwneud â'i ddramâu llwyfan, [1966]-1992, a'i ddramâu teledu, radio a ffilm, [1966]-[1991]; papurau'n ymwneud ag addasiad teledu Gwenlyn Parry ac Endaf Emlyn o nofel Caradog Prichard, Un Nos Ola Leuad, [1966]-1991; sgriptiau gweithiau gan eraill, [1966]-1991; papurau amrywiol yn ymwneud â'i waith, megis rhageiriau ac erthyglau, 1968-[1991]; deunydd printiedig, 1962-1991; a phapurau personol a theyrngedau, 1962-1993. = Papers of Gwenlyn Parry, [1962]-1993, comprising scripts and various papers relating to his stage plays, [1966]-1992, and television and radio dramas, [1966]-[1991]; papers relating to Gwenlyn Parry and Endaf Emlyn's television adaptation of Caradog Prichard's novel Un Nos Ola Leuad, [1966]-1991; scripts of works by others, [1966]-[1991]; various work-related papers, such as prefaces and articles, 1968-[1991]; printed material, 1962-1991; and personal papers and tributes, 1962-1993.

Papurau'r bardd Tydfor Jones, [1931]-1993, yn cynnwys ei gerddi cynnar, cerddi'r gyfrol Rhamant a hiwmor a Tydfor a gyhoeddwyd yn 1993, ynghyd â phapurau'n ymwneud â Bois y Cilie, yn arbennig ei ewythr John (Tydu) Jones a ymfudodd i Ganada. = Papers of the poet Tydfor Jones, [1931]-1993, comprising his early poems, poems for Rhamant a hiwmor a Tydfor published in 1993, together with papers relating to Bois y Cilie, especially his uncle John (Tydu) Jones who emigrated to Canada.

Papers of artist, lecturer, curator and writer Moira Vincentelli, comprising material relating to the 1985 Women's Art in Wales touring exhibition and to other exhibitions; questionnaires completed and returned by Welsh women artists and craftspeople; material relating to the 1983 Retrospective Exhibition by painter and poet Ray Howard-Jones; general correspondence; and miscellaneous material.