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Eighteen diaries and notebooks containing memoranda and accounts by Howell Vaughan, 1663, Katherine, widow of Griffith Wynn of Bodfean, and later wife of Colonel Hugh Nanney, 1692, Hugh Evans, agent to the said Katherine, 1682-1690, Lumley Williams of Ystumcolwyn, 1696, Robert Vaughan of Hengwrt, 1745 , and others.
Several of the diaries, which include almanacks by Trigge, Gallen, and Rider and the Daily Journal, contain entries relating to the Nannau estate. Rider's British Merlin for 1698 contains a few englynion in manuscript, and in one notebook there are inventories of linen and utensils at Nannau, 1692.

A facsimile manuscript in two parts mostly in the hand of William Watkin Edward Wynne. The first part comprises copies (some printed) of charters, public records, deeds, pedigrees, poetry, etc. of Merionethshire and Caernarvonshire interest, some of which are taken from transcripts made by Robert Vaughan, Hengwrt. The material includes records and pedigrees relating to the Wynn family of Peniarth; notes on the Maurice and Owen families of Clenennau, Penmorfa, Caernarvonshire, with related deeds possibly in the hand of William Maurice of Llansilin; deeds relating to the Porkington estate; an extent of the commote of Eifionydd, 1352; an extract from the Coroner's Rolls for Merionethshire, 1345; charters of Castell y Bere and Harlech Castle; pedigrees of Madog ap Dafydd of Hendwr, Llandrillo, Merionethshire; an ode to Einion ap Gruffydd of Corsygedol by Gruffudd Gryg; odes to Dafydd ab Ieuan ab Einion by Guto'r Glyn and Dafydd Nanmor; letters addressed to W. W. E. Wynne, the correspondents including Walter Davies ('Gwallter Mechain'); etc. The second part is also mostly in the hand of W. W. E. Wynne and again comprises material mainly of Merionethshire and Caernarvonshire interest, including pedigrees, correspondence, deeds, etc. relating to the Porkington estate and to the Maurice family and to the Wynne family of Glyn and Ystumcegid, Caernarvonshire; poetry relating to members of the Wynn family of Glyn by Huw Machno, Rhisiart Cynwal and others (one elegy translated into English); press cuttings taken from the Cambrian News, 1879; letters addressed to W. W. E. Wynne, the correspondents including Walter Davies ('Gwallter Mechain') and Joseph Morris; etc.

Facsimile of letters, 1601-1738, mainly of the Owen family of Peniarth and the Nanney family of Merionethshire. The correspondents include Lewis Owen (1625-1691); Richard Owen (d. 1714); Lewis Owen (d. 1729), son of Richard Owen; Elizabeth Owen, mother of the latter Lewis Owen; Margaret Owen, wife of the latter Lewis Owen and daughter of Sir William Williams, second bart, of Llanforda; Jane Bulkeley (d. 1765), daugher of Lewis and Margaret Owen; Hugh Nanney; and Richard Nanney. Other correspondents include Robert Vaughan, Hengwrt, and there are letters from Margaret Owen to her father, Sir William Williams.
There is an introductory note by William W[atkin] E[dward] Wynne at the beginning of the volume, which states that "all the letters addressed to Sir William Williams, Bart., were found in the muniment room at Wynnstay, and were given to me ... in October 1833 by the Rt Honble C. W. Williams Wynn". There is a reference in the note to Dr Samuel Johnson in relation to the education of girls and women.

Transcripts by Robert Vaughan of tracts and documents relating to the Council in the Marches of Wales, including 'The Inconveniences of exemptinge English sheires [Gloucester, Worcester, Monmouth, and Salop], shewed to Queen Elizabeth'; propositions concerning the jurisdiction of the King's Bench in the Marches; precedents for installing plaintiffs in possession; 'The effecte of the King's speech ... 3 November 1608'; 'A Treatise of Wales and the Marches thereof'; an abstract of records in the Tower concerning the Marches; 'A discourse or relation of the ancient and moderne estate of the Principalitie ... by Serieant Dodderidge'; instructions to the Council of the North, 1595/6; a survey of lands in Tal y Bont, Merioneth; a note on the lordship of Glasbury; and 'A description of the Councell and Court established in the Principality and Marches of Wales', and 'An exemplification touching proceedings in Chancery at the request of ye right honorable Ralphe Lo: Eure'.

Transcripts, mainly by Robert Vaughan, Hengwrt, of the extent of the lordship of Denbigh, 8 Edward III; an exemplification of letters patent granted to John Weston, prior of the Hospital of St John of Jerusalem, 7 Henry VII; an undated extent of Merioneth; accounts of the escheator of Merioneth, 1615; and the extent of Caernarvon, 26 Edward III. Ff. 131-134 are very fragmentary.

A collection of transcripts, mainly by Robert Vaughan, Hengwrt, of records relating to North Wales, including the extent of North Wales by John de Delves, 26 Edward III; a record of a view of frankpledge for the commote of Menai, 28 Henry VIII; ministers' accounts for Flintshire, 30-31 Henry VIII; extracts from miscellaneous inquisitions, rentals, court rolls, and correspondence; receipts of Lewis Owen, deputy receiver of North Wales, 1 & 2 Philip and Mary; notes of leases under the exchequer seal, 1579; notes on the form of administration of justice in Wales by Auditor Hill; 'The State of the Dominion of Wales' by Sir Thomas Canon; accounts of John Lloyd of Ragad, escheator of Merioneth; instructions to the Earl of Bridgewater, President of the Council in Wales and the Marches, 1633; a roll of the coroner for Merioneth, 10-11 Edward III; estreats of fines in North Wales, 22-30 Edward III; lists of persons indicted in Merioneth, 6- 19 Richard II; records of pleas before the justice of North Wales, 4 Edward II; a list of recognisances in the exchequer at Caernarvon, 18 Edward II; lists of persons in Anglesey fined for being in arms with Owen Glyndyfrdwy, with lists of outlaws and jurors; and a breviate of an account between Sir John Salesbury, chamberlain of North Wales, and Lewis Owen, his deputy, 1555.

Transcripts by Robert Vaughan, Hengwrt of the Vitae duorum Offarum of Matthew Paris (the concluding paragraph only of the first Offa), and of a history of Wales entitled 'liber primum de Cambriae regimine bellico, sub Principibus Britannico sanguine aeditis'.
The latter is an incomplete copy of the first book of a projected treatise in three books.

A volume of papers from the Mytton library at Halston, consisting of draft dissertations by Dr. Humphrey Foulks of Marchwiel and other papers:- 'a dissertation of the literature of the antient Britains'; 'a dissertation on the places of worship, judicature, and sepulture of the antient Britains'; 'a short dissertation on the state of the lordship of Denbigh'; 'an essay about the setting of land'; a fair copy of a preface to 'The modern Antiquity of Wales'; a draft title-page and preface to a projected edition of Robert Vaughan's British Antiquities Revived, and Sir John Wynn's 'History of his own family'; drafts and transcripts of letters and documents relating to Welsh history; transcripts from 'Mr. Owen Salisbury's painted book'; transcripts of annals of the rebellion in North Wales; pedigrees; lists of the sheriffs of Flint and Denbighshire to 1739, extended by another hand to 1741; transcripts of monumental inscriptions in Bangor [on Dee], Wrexham, Gresford, Marchwiel, and Montgomery; a valor of Bromfield and Yale, 11-12 Henry VIII; and holograph letters by Rees Powell, Llanharan, 1736, Thomas Lewis, St. Asaph, 1736, and E. Lloyd, Ripple, 1737.

A transcript of Robert Vaughan of Hengwrt's essay, printed Oxford, 1662, under the title British Antiquities Revived: or a friendly Contest touching the sovereignty of the three Princes of Wales in ancient times ... .

A miscellaneous collection of records mainly relating to Wales compiled towards the middle of the seventeenth century. -- The manuscript begins on page 53 with extracts from 'Llyfr Coch Asaph', with the additions from the hand of William Bullocke, as in Peniarth MS 231 - a manuscript written by Robert Vaughan, Hengwrt, and most probably the immediate source of the Nefydd version; the 'summa' of 'Llyfr Coch Asaph' compiled in 1602, which is also contained in Peniarth MS 231, as well as the list of contents of another St. Asaph record - the 'liber pergamenus' which is now deposited with the Church in Wales records at the National Library; a transcript of a record of proceedings on a writ of quare impedit brought by the Prince of Wales against Howel Gymen and a hundred and seventeen others, touching the advowson of a prebend in the collegiate church of Holyhead ('prebenda de Castro Keby') supplied by 'Mr. Ellice the Councellor'; a collection of historical records relating to Wales taken directly from the hand of Robert Vaughan in Peniarth MS 236; a transcript of the 'Historia Britonum' of Nennius, copied out of a book given to John Selden by William Camden, compared with a version in 'Oxford Library' under the name of 'Gilda Minor', and ending with an extract from a Cottonian manuscript (pp. 245-88); a copy of the statutes of Chester Cathedral, temp. Henry VIII (pp. 289-310); 'Ymrafaelion henwau Ynys Brydain', etc. - seventeen chapters of pseudo-history and description of the Isle of Britain (cf. slightly different versions in Peniarth MSS 163 and 215), with a supplement containing accounts of place-names not included in the main text, a reference to the earthquake of 1574/5, the wonders of Scotland and Ireland, the conversion of the various British nations to Christianity, and 'y naw helwriaeth', 'mesurau cerdd dant', and 'trioedd mab y krinwas' (pp. 312-49). -- At the end of the volume are a number of documents relating to Cheshire and Flintshire - a note of entail of Flintshire lordships, Flintshire rents of assize, the customs of Dee mills and other records taken from a book of Edward Whitby, recorder of Chester, and a transcript of Robert Vaughan's copy of the fealty roll of the Prince of Wales, 29 Edward I .

A volume containing texts of (a) the fuller version of 'Ystoria Dared' (pp. 1-40), translated by Peter Roberts in The chronicle of the Kings of Britain, 1811, (b) the so-called 'Brut Tysilio' or 'compiled version' of Geoffrey of Monmouth's 'Historia Regum Britanniae' (pp. 41-198), also partly translated by Peter Roberts (op. cit.), and closely allied to the text of British Museum MS Cotton Cleopatra B.v., and (c) 'Brut y Saeson' to the year 1461 (pp. 199-308). Pp. 1-88 are in a late 14th century hand; the remaining pages are in the hand of Gutun Owain, the 15th century bard and herald associated with the abbey of Basingwerk. A note, dated 1630, by Robert Vaughan, Hengwrt refers to the misplacement of many pedigrees, and another note, dated 1809, by Peter Roberts refers to the identification of the volume by William Maurice, Cefn-y-braich.

An autograph letter, 7 February [16]93, from Humphrey Humphreys, bishop successively of Bangor and Hereford (1648-1712), to Peers Maudit, Windsor Herald; letters and genealogies sent to Bishop Humphreys, 1704-1707, by Peter Le Neve, Norroy King of Arms (1661-1729), and Thomas Humphreys, mainly concerning the pedigree of Sir William Humphreys, a sheriff of the City of London, with notes thereon and on Robert Vaughan, Hengwrt (1592?-1666), by Bishop Humphreys.

Transcripts, begun in 1683, of Sir John Wynn, History of the Gwydir Family taken from 'a Coppy belonging to Sr Morris Parry of Llan Elian Clerk, in the year 1674 and afterwards compar'd with & corrected by two Coppys, the one Belonging to the Reverend Dr Humphreys Dean of Bangor, the other found among the Evidences att Gwedir, which last was in many places corrected & interlin'd, & much of it writt with the hand of Sr John Wynn himselfe the author'; 'Ystoria Gruffudd ap Cynan ...' copied for Thomas Mostyn, Gloddaeth, 1683, from 'Llyfr Plas-y-ward'; 'a chronicle supos'd to be collected by Robert Vaughan of Hengwrt ...'; charters, indentures, petitions, etc.

Three Welsh Grammars; The Dream of Maxen Wledig; Elucidarium; Commotes and Cantreds of Wales; Astronomi; etc., mainly in the hand of Thomas Williams before he began to sign himself 'Thomas ap Wiliam physicwr'. Pages 112-114 and 129-130 are in the autograph of Robert Vaughan of Hengwrt, 16th May 1656, and Darogan Beli (p. 216) appears to be written by D. Jones (?o Lanvair Dyffryn Clwyd).

A volume in the hand of Evan Evans (Ieuan Fardd) containing a transcript of an address to Robert Vaughan of Hengwrt by William Maurice, 1661 (ff. 1-46); and a Catalogicus Chronologicus Scriptorum Britannicorum (ff. 46 verso-52); etc.

Five booklets containing transcripts by Evan Evans (Ieuan Fardd), including a commonplace book of Dr Thomas Williams; letters to Edward Lhuyd from Sir Richard Mostyn, John Tibbots and others; letters from Humphrey Humphreys to Lewis Anwyl; 'Trioedd Ynys Prydain' with notes by Robert Vaughan, Hengwrt [possibly related to NLW MS 2019C] (ff. 49-70); various texts written by Thomas Williams and Robert Vaughan; a Welsh-English vocabulary; pedigrees; etc.

Twelve booklets containing transcripts, [1772x1787], by Evan Evans (Ieuan Fardd) from various printed and manuscript sources relating to the history of Wales, including letters from Dr John Davies of Mallwyd to Sir John Wynn and Owen Wynn of Gwydir in relation to Dr Thomas Williams's dictionary; letters from Robert Vaughan to Sir Richard Wynn and Sir Owen Wynn; an account of Merioneth by Robert Vaughan; 'Cywydd marwnad Huw Morus'; and a 'carol plygain' by Edward Samuel.
Transcribed in part from a book published in MDCCLXXII [1772] (p. 6).

A composite volume mostly in the hand of Evan Evans (Ieuan Fardd) containing a copy of Sir John Wynn's History of the Gwydir Family, taken from a transcript made by Thomas Mostyn of Gloddaith (ff. 1-74); extracts from papers of Robert Vaughan, Hengwrt (ff. 75-86); lists of manuscripts at Gwydir and Llannerch (ff. 89 verso-94, 185) (for the Llannerch manuscripts see Cambrian Register, Vol. i, p. 320, etc.); poetry by Siôn Cent, Tudur Aled, Siôn and Gruffydd Phylip and others (ff. 95-153, 190-203); a pedigree of the Panton family (ff. 186-189); copies of letters from Edward Lhuyd to Robert Davies, Llannerch (ff. 204-219), and of a letter from Thomas Price, Llanfyllin to Robert Davies, Llannerch (ff. 220 verso-225); extracts; etc.

A composite volume mostly in the hand of Evan Evans (Ieuan Fardd) containing transcripts of correspondence between Lewis Morris, Edward Richard, James Phillips and Samuel Pegge (see Cambrian Register, Vol. i, p. 357) (ff. 1-36); a copy of Morgan Jones's letter from New York, 10 March 1685/6, relating to Welsh Indians (ff. 41-43) (see the Gentleman's Magazine, 1740, and NLW MS 2577B); extracts from a letter of Griffith Roberts (ff. 54-57) and from a commonplace book of Robert Vaughan, Hengwrt (ff. 193-208); proverbs in Welsh and Latin (ff. 58-63); autograph proposals for printing a book of poetry (later 'Gorchestion Beirdd Cymru') to be edited by Ieuan Fardd and Rhys (Rice) Jones and published by David Jones, Trefriw (ff. 89-92); a note on manuscripts in the Mostyn library (ff. 98-99); a copy of Henry VII's charter of North Wales (f. 100); poetry (ff. 112-113, 116-124, 209-212); the Introduction to Lewis Morris et al's Celtic Remains, and copies of letters from Lewis Morris to Robert Vaughan and others (ff. 125-164); a copy of Annals of Wales by Robert Vaughan (ff. 165-192) (see Mostyn MS 136); chronicles, etc. with notes by Lewis Morris (ff. 213-239); further extracts from various sources; etc.