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Electoral lists of the commotes of: Ardudwy Uwch Artro, 1860-1861; Ardudwy Is Artro, 1861; Mawddwy, [1860s]; Tal-y-bont, 1861-1863; and Ystumanner, 1860; and jury lists for the parishes of Beddgelert; Dolgellau; Llanfihangel-y-Pennant; Llanfihangel-y-traethau; Llanfrothen; Llangelynnin; and Trawsfynydd, 1866.

Deeds and documents of the Bennett family of Glanyrafon, Montgomeryshire, and the Owen family of Dolgoed and Llawrpenegoes, 1546-1946, relating mainly to properties in the parishes of Llanidloes, Llanwrin, Penegoes, and Trefeglwys, Montgomeryshire, and Talyllyn, Merionethshire; and a map of properties in Trefeglwys, 1819.

Deeds, 1490-1977, including deeds and documents mainly relating to properties on Anglesey, Caernarfonshire, Merionethshire and Middlesex, 1675-1977; and deeds relating to properties in Finchley, Middlesex, 1490-1796.

Personal papers of Sir John Williams comprising notes, essays, lectures and transcripts by him, [19th century]-[early 20th century]; certificates and testimonials, 1858-1915; cards and letters from the children of King George V and invitation cards to royal functions, 1889-1916; documents relating to his various honours, 1894-1911; photograph and stamp albums, 1849-[early 20th century]; other photographs, [1840s]-1905; press cuttings, [c. 1870]-1926; letters collected by Sir John, 1633-1912; letters to him, 1879-1922, the correspondents including members of the Royal Family; deeds and other documents relating to properties in Llangadog, to Plas Llanstephan and to Harley Street, London, 1790-1918; bibliographical material, [19th century]-[20th century]; medical notebooks and other papers, 1855-1900; diaries of Sir John and Lady Williams, 1872-1925; estate and financial records, 1890-[1926]; papers relating to public affairs, 1870-1911; miscellaneous items collected by Sir John, 1795-[c. 1919]; personal possessions, including University and commemorative medals, insignia, medical equipment, and ceremonial trumpets, 1861-1913; and deeds collected by Sir John Williams, 1546-1869, comprising deeds of the Vaughan family of Llanelli, Carmarthenshire, the Penry family of Swansea, Glamorgan, and the Dalton family of Pembrey, Carmarthenshire, 1545-1677, relating to properties in Llangennech and Pembrey, Carmarthenshire; deeds of John Jones, Ystrad, Carmarthenshire, relating to Llansadwrn, Carmarthenshire, 1632-1793, and the borough of Carmarthen, 1611-1869; Wynn of Gwydir deeds, 1352-1797, relating mostly to Caernarfonshire, Merionethshire and Denbighshire; miscellaneous Welsh deeds, relating mainly to properties in Carmarthenshire and Cardiganshire, 1451-[c. 1840]; and miscellaneous deeds relating to England (mainly Cornwall and Staffordshire), Ireland, and Scotland, 1586-1896.

Papers, 1679-1983, of and accumulated by H. Noel Jerman, comprising: research papers, 1914-1975; files relating to his work in the Secret Intelligence services, 1941-1945; correspondence, notes and other papers relating mainly to archaeology, and also to his professional activities, 1948-1983; 'Notes and Memoranda' relating to events organised by the Cambrian Archaeological Association, 1883-1894; original records collected by him, 1679-1926, including deeds and documents relating to properties in Kerry, Montgomeryshire, 1679-1885, and Kerry School, 1843-1873, and copies of local newspapers, 1834-1868; records relating to the Dolforgan estate, including deeds and documents relating to properties in Montgomeryshire, Carmarthenshire and Merionethshire, 1807-1910, financial records, 1889-1939, and letter books, 1892-1930.

An additional consignment of materials of, and accumulated by, the late H. Noel Jerman (1909-1994), including his research papers relating to properties in Kerry and surrounding areas, papers relating to the Dolforgan estate, together with maps, sale catalogues, plans and photographs, and a lithograph of Dolforgan Hall by T. Way. This group remains uncatalogued.

Ledger and journal of Gaewern Slate works, Machynlleth, 1835-1856; accounts and notebooks of the Ratgoed and Cymerau Slate Quarries, Tal-y-llyn, and Llwyngwern Slate Quarry, Llanuwchllyn, 1853-1899; ledgers and notebook of the Cambrian Slate Works, Machynlleth, 1899-1909; minute books of the Abercorris Slate Quarry Company, Rhiwgwreiddyn, Corris, 1893-1909, and the Towyn Company, Tywyn, 1893-1903; and miscellaneous accounts and ledgers, 1827-1909.

Deeds, documents and probate records, 1617-1853, relating mainly to the parishes of Caerhun, Conwy, Dwygyfylchi, Gyffin, Llanbedrycennin and Llannor, Caernarfonshire, and to the Abbey estate, in Denbighshire, Merionethshire and Caernarfonshire, 1811-1819; notes on sermons, 1861-1889; and miscellaneous papers relating to Amlwch, Anglesey, 1801-1868.

Deeds and documents, 1598-1856, mostly assignments of mortgage and related bonds, concerning Dôl y Cae and other premises in the parish of Tal-y-llyn, including a lease from William Owen Pughe and his brother Richard to his son Aneurin Owen Pughe.

Papurau Arthur Cadnant Ellis [20fed ganrif], yn cynnwys traethodau ar 'Rhai o Enwogion Aberllefenni' a 'John Jones (Jac) Glan-y-gors a'i Amserau (1766-1821)'; braslun o hanes achos y Methodistiaid Calfinaidd yn Harlech a Llanfair, sir Feirionnydd; torion erthyglau, llythyrau, etc., a gyfrannodd i'r wasg; a nodiadau amrywiol = Papers of Arthur Cadnant Ellis, [20th century], including essays on 'Rhai o Enwogion Aberllefenni' and 'John Jones (Jac) Glan-y-gors a'i Amserau (1766-1821)'; a brief history of the Calvinistic Methodist cause in Harlech and Llanfair, Merionethshire; cuttings of articles, letters, etc., which he contributed to the press; and miscellaneous notes.

Papers of the Pale estate belonging to Henry Beyer Robertson, 1879-1950, comprising correspondence on Council matters, especially the contract between Bala Urban District Council and Merionethshire County Council for the upkeep of the main roads, 1880-1948; pamphlets, diagrams and letters concerning the Pale hydro-electric plant, 1892-1936; and miscellaneous papers, 1885-1948, including items relating to the 1885 general election campaign in Merionethshire.