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Research notes and a draft catalogue of the worksheets of In Parenthesis and The Anathemata by David Jones compiled at the Library in 1981, together with a list of letters by Tony Stoneburner, 1977, a catalogue of parts of the archive by Harman Grisewood, and a Catalogue of the artist's drawings and papers in the possession of the David Jones Trustees in 1992, prepared by Matilda and Douglas Hall.

This collection comprises forty petitions submitted by various ratepayers and parishes to county magistrates, expressing both opposition to and support for the proposed erection of a joint "lunatic asylum". Included are printed agreements concerning the establishment of the asylum, along with correspondence regarding the proposed site. A letter from the Clerk of the Peace Office in Stafford is accompanied by a county's asylum map layout . The collection also contains several drafts of meeting minutes, letters, and attendance records related to the proposed joint asylum for the counties of Carmarthen, Cardigan, Glamorgan, and Pembroke. the collection also includes a draft agreement dated 17 June 1847, approved by committees, for the union of Carmarthen, Glamorgan, and Pembroke for the construction of the asylum, followed by a formal agreement dated 4 August 1847. Additionally is a that bundle that contains draft agreements for the sale and purchase of land in the parishes of Swansea and Llansamled, including a 1000-year lease of the Danygraig Fawr estate in Glamorgan. There are also Legal documents titled case for the opinion of Mr. E. R. Williams on the interpretation of clauses 8 and 9 of 9 Vic. c.126, and the response of William Llewellyn to a bill of complaint filed by John Austin on 22 March 1861.

Also included are notes of lectures delivered by Professor Jac L. Williams in Malta and Yugoslavia.

Papers relating to the centenary of the restoration of St David's Church, Bettws. (Facsimilies of Church in Wales records of 1684.) English. Buckram. Donated by the Reverend D. F. Donald Jones, Ammanford, February 1971.

Papers, 1914-1930, relating to the establishment of the Central Welsh Board, including reports, minutes, letters and auditor's reports.

Correspondence and other papers, 1895-1915, including receipts from the Copyright Office, Library of Congress, Washington, relating to musical compositions deposited by the composer David Jenkins, and a few from the British Museum. There is a note, 1944, in Welsh, from T. G[wynn] J[ones] to the composer's niece, regarding these papers.

Papers relating to the Dongray estate by William Fowler Jones and others. In boards. Donated by John L. Hobbs, F.L.A., Shrewsbury, January 1950.

Papers relating to the Eisteddfod held under the auspices of the Lanka Cambrian Society, Colombo, including some of the compositions; a booklet relating to the event, 'Braslun o hanes Eisteddfod Lanca 1945', compiled by Wyn Jones; and copies of the monthly newsletter of the society. cf. NLW MS 14811E and Minor Deposit 1361B.

Papers relating to the election of 1935 in the Carmarthen Parliamentary Constituency and to the appointment of a counting assistant. English. Between boards. Donated by the late T. J. Evans, Esq., M.B.E., Clunderwen, February 1966.

Papers relating to the experiment to introduce bilingual education at the Cilfynydd Boys' Council School, Pontypridd, co. Glamorgan between 1930 and 1936, under the supervision of John Phillips, the headmaster.

Papers, photographs and memorabilia relating to the Festival of Wales, 1958. Sir Clayton Russon (1895-1968) was the President of the Festival and included are two telegrams from HM Queen Elizabeth II.

Original copies of the opinions of people from all parts of Wales towards the 2005 G8 Summit. The papers were collected by the donor during three months travelling around Wales on her bike, named as the Blossom Bike Tour.

Papers relating to the General Annual Licensing Meeting, Petty Sessional Division of Llanelli, co Carmarthen, 9 Feb 1921, including applications for new licences and agenda of cases.

A copy of the National Archives's file, HO 144/22915, relating to the growth of the Welsh National Movement in Wales and how to use the royal family in order to try to impede this, 1939-1941.

A volume containing copies of the correspondence, 1997, between former Secretary of State Ron Davies and former Cardiff Council Leader Russell Goodway with regards to the home of the National Assembly for Wales, and papers relating to the possible future use of Cardiff City Hall by the Welsh Assembly Government.

Research papers collated by Peter N. Williams for his research on David Thomas known as 'Father of the American Anthracite Industry', who emigrated to Pennsylvania in 1828 from Ystradgynlais, including letters from a collection held at the Hagley Museum & Library, Wilmington, Delaware.