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The collection comprises mainly leaflets, correspondence and papers, 1924-1966, relating to Labour politics in the Brecon and Radnor constituency. There are also papers concerning the Labour Party in Wales, 1928-1952; the Parliament for Wales campaign, 1950-1956; Tudor Watkins's visits to Russia in 1961 and to Patagonia in 1965; papers concerning Tudor Watkins's elevation to the House of Lords in 1972; and material deriving from the Brecon and Radnor by-election in 1939.

Papers of Lord Ystwyth, 1895-1920, including Cardiganshire Liberal Association minutes of meetings, accounts, bills and receipts, and correspondence of Lord Ystwyth, 1907-1921; papers relating to the establishment and activities of the Cardiganshire Battery, 2nd Welsh Brigade, Royal Field Artillery, 1897-1913; and tickets of admission to events in Aberystwyth, 1898-1904.

Papers of the Breton nationalist Louis Feutren (1922-2009), together with papers of two fellow nationalists accumulated by him, Neven Henaff (Célestin Lainé, 1908-1983), and Alan Heusaff (1921-1999). All three were prominent members of the Breton collaborationist force 'Bezen Perrot' formed in December 1943, and all three eventually fled to Ireland sometime after the Second World War. Some of the papers relate to the activities of 'Bezen Perrot', but most are later personal papers.

Lower Swansea Valley Project Report I: 'The Human Ecology of the Lower Swansea Valley' by Margaret Stacey (cyclostyled). English. Boards. Donated by Hugh O'Neill, University College, Swansea, May 1967.

Lower Swansea Valley Project Report II: 'Transportation and Physical Planning in the Lower Swansea Valley' by R. D. Worrall (cyclostyled). English. Boards. Donated by Hugh O'Neill, University College, Swansea, May 1967.

Lower Swansea Valley Project Report III: 'Report on the Hydrology of the Lower Swansea Valley' by D. C. Ledger (cyclostyled). English. Boards. Donated by Hugh O'Neill, University College, Swansea, May 1967.

Lower Swansea Valley Project Report IV: 'Final Report on the Geology of the Lower Swansea Valley Project Area' by W. F. G. Cardy (cyclostyled). English. Boards. Donated by Hugh O'Neill, University College, Swansea, May 1967.

Lower Swansea Valley Project Report IX - reports on plant ecology: 'Vegetation Trials' by R. L. Gadgil; 'Large Scale Grass Trials' by L. J. Hooper & R. G. Jones; 'Soils' by E. M. Bridges.' English. Boards. Donated by Hugh O'Neill, University College, Swansea, May 1967.

Lower Swansea Valley Project Report V: 'The Soil Mechanics and Foundation Engineering Survey of the Lower Swansea Valley Project Area' by H. G. Clapham, H. E. Evans, & F. E. Weare (cyclostyled). English. Boards. Donated by Hugh O'Neill, University College, Swansea, May 1967.

Lower Swansea Valley Project Report VI: 'The prospects for Industrial Use of the Lower Swansea Valley - A Study of Land Use in a Regional Context' by Susanne H. Spence (cyclostyled). English. Boards. Donated by Hugh O'Neill, University College, Swansea, May 1967.

Lower Swansea Valley Project Report VII: 'Lower Swansea Valley Housing Report' by Margaret Stacey (cyclostyled). English. Boards. Donated by Hugh O'Neill, University College, Swansea, May 1967.

Lower Swansea Valley Project Report VIII: 'Lower Swansea Valley Open Space Report' by Margaret Stacey (cyclostyled). English. Boards. Donated by Hugh O'Neill, University College, Swansea, May 1967.

Lower Swansea Valley Project Report X: 'Soil Biology of the Lower Swansea Valley' by P. D. Gadgil (cyclostyled). English. Boards. Donated by Hugh O'Neill, University College, Swansea, May 1967.

Lower Swansea Valley Project Report XI: 'Afforestation of the Lower Swansea Valley' by B. R. Salter (cyclostyled). English. Boards. Donated by Hugh O'Neill, University College, Swansea, May 1967.

Lower Swansea Valley Project Report XII: 'Tips and Tip Working' by G. Holt; 'Estimation of Quantities of Materials' by H. E. Evans; 'Preliminary investigation of creating an artificial lake' by R. E. Davies (cyclostyled). English. Boards. Donated by Hugh O'Neill, University College, Swansea, May 1967.

Deeds, 1856-1946, relating to the Holyland estate of the Adams family in Pembrokeshire.

Fine book, 1872-1921 of the Loyal Iolo Goch Lodge of Oddfellows, Tal-y-bont, Cardiganshire.

Balance sheets, 1877-1934, of the Aberystwyth Loyal Temple of Love Lodge of Oddfellows. Two photographs, [?1911], and a bond, dated 1879, were added in 1997 and 1999 respectively.

One of six night books, 1875-1908, showing payments of sickness benefit made by the Aberystwyth Loyal Temple of Love lodge of Oddfellows.

One of six night books, 1875-1908, showing payments of sickness benefit made by the Aberystwyth Loyal Temple of Love lodge of Oddfellows.