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A composite volume consisting of two incomplete manuscripts written by several mid-seventeenth century scribes and containing Welsh poetry mostly in strict-metre.
It comprises: (a) pp. 1-498, 595-622 (many misplaced leaves, the original order being pp. 615-616, 179-186, 37-38, 595-598, 619-622, 599-602, 35-36, 1-34, 39-178, 187-432, 603-614, 433-498) mainly in the hands of Richard Cynwal (pp. 37-38, 179-186, 615-619) and an unidentified mid-seventeenth century scribe, containing Welsh poetry addressed mostly to the Maurice family of Clenennau and related families, including those of Bryncir; Wern, Penmorfa; Craflwyn, Beddgelert; Ystumcegid and Corsygedol; (b) pp. 499-594 in the hand of an unidentified mid-seventeenth century scribe, containing Welsh poetry addressed to families of north-east Wales, particularly those of Eutun of Leeswood and Lloyd of Bodidris. Poems, probably holograph, by Ellis Rowland, Jane Vaughan of Caer Gai and William Wynne are tipped in at the end of the volume (pp. 623-625).

A composite manuscript of loose papers and fragments of manuscript volumes. It contains poetry and prose, mostly in Welsh, much of the poetry being addressed to the Owen family of Brogyntyn and Clenennau and other related families. Apart from a late-sixteenth century awdl by Wiliam Llŷn (ff. 57-58), the other items all belong between the first half of the seventeenth century and the first half of the eighteenth century.
Fragments apparently once part of books, some of which perhaps were never bound, are: a narrow folio of cywyddau and englynion by Mathew Owen, in the hand of Nathanael Jones (ff. 20-26), written not before 1656 (see ff. 24 verso-25), with autograph englynion added by Harri Howel (f. 20 verso) and by Nathanael Jones (f. 20 verso, 23); a folio manuscript containing cywyddau to Lewis Anwyl of Parc and his family, dated 1627-1636 (ff. 38-55), written by two good hands of the first half of the seventeenth century, one responsible for ff. 38-50 verso, the other ff. 51-55; a quarto manuscript with transcripts of poetry of the Gogynfeirdd (ff. 113-122; paginated 1-20), by a seventeenth-century hand similar to that of Morris Evans (cf. ff. 93-94, 123-141); pedigrees of Welsh royal lines, the Maurices of Clenennau, etc., in English (ff. 123-141; original foliation 1-12 survives), in the hand of Morris Evans (ff. 123-127 verso, 129-134 verso) and a second hand (ff. 128 recto-verso, 135-141); a narrow folio of canu brud attributed to Myrddin, Taliesin, etc. (ff. 178-186), written by Nathanael Jones, not before 1651 (ff. 182 verso, 183 verso 'aetatis suae a 21o Feb: 1650 27'); a folio manuscript of canu brud, mainly cywyddau, by Dafydd Llwyd and others (ff. 189-207), in a poor hand of the mid seventeenth century, probably that of Thomas Edwards to judge by pentrials on f. 196 verso, who refers to Tregeiriog (f. 199 verso) and 'Llanfylling fairings' (f. 207 verso); an octavo manuscript containing poems by Robin Clidro, etc., in a seventeenth or eighteenth century hand (ff. 210-219); and a folio manuscript of autograph cywyddau and englynion by Huw Morys, some addressed to William Owen and Sir Robert Owen (ff. 222-226 verso). Poetry written on loose papers includes autograph poems by Huw Morys (ff. 12-18), John Owens (ff. 59-71; f. 69 recto-verso may be his italic hand), Harri Howel (ff. 75-76 verso, 90 recto-verso), Owen Gruffydd (ff. 84-89, 230-231), William Phylip (ff. 97-98 verso), John Morgan, later vicar of Conwy (f. 101 recto-verso, the poem incomplete and anonymous, dated 1688, the hand his), Siôn Rhydderch, 1732 (ff. 104-105, 227-228), and Edward Lloyd, Brewis (f. 221 recto-verso). There are probable autograph poems by Edward Rowlant (ff. 72-74 verso, 79-80) and John Richard (f. 81), and possible autograph poems by 'J. Ll.' (f. 26 verso), Mathew Owen (ff. 77-78, 232 recto-verso), Siôn Roberts (ff. 91-92), Huw Cadwaladr (ff. 106-108) and 'R.C.' (f. 163). Other poetry is in the hands of Morris Evans (ff. 93-94) and 'Theo: Ro:' (ff. 152-154 verso). Also included is a letter, 1652, from the antiquary Meredith Lloyd to Thomas Vaughan, the alchemist and poet (ff. 1-3 verso), followed by a copy of Hanes Taliesin (ff. 5-10 verso). The 'Cywydd Marwnad i Mr William Owen o Borkynton' by Huw Morys, beginning 'Mae gwaedd oer lem Gweddw [yw'r wlad]', discussed in E. D. Jones, 'The Brogyntyn Welsh Manuscripts', National Library of Wales Journal, 7 (1951-2), 165-198 (pp. 186-189, 196-197), has not been found.

Records of the Brogyntyn estate, home of the Ormsby-Gore family, Barons Harlech, 1296-1951. They include estate papers and deeds, legal papers, financial papers, family papers and county administration papers of the Ormsby-Gore family, their ancestors, the Maurices and the Owens of Clenennau, the Wynns of Glyn and others, such as Anwyl of Park, Clayton of Lea Hall, Godolphin of Abertanat, Lyster of Penrhos, Mostyn of Nant, and Vaughan of Corsygedol. The three main estates represented in the collection are Brogyntyn, Clenennau and Glyn, the latter constituting a major addition to the existing North Wales holdings of Sir Robert Owen upon his marriage to Margaret Wynn in 1683. The documentation also covers other, subsiduary estates acquired by marriage or inheritance, namely Llanddyn, Sylfaen, Ystumcegid, Nant, Cemais, Penrhos, Abertanat and properties in the west of Ireland. The record types include title deeds for lands in Caernarfonshire, Merionethshire, Flintshire, Denbighshire, Montgomeryshire, Shropshire, elsewhere in England and Wales, and in the Irish counties of Westmeath, Leitrim, Sligo, Mayo and Roscommon, 1296-1838; rentals, accounts and other papers associated with estate administration, [1380s]-1951; manorial records, 1429-1804; household management papers, 1662-[c. 1949]; legal and arbitration papers, 1410-1834; financial papers such as mortgages and accounts, 1492-1876; family settlements, probate records and trusts, 1485-[c. 1862]; private letters, 1582-1950; papers relating to family interests, [14th cent.]-1951; personal papers of family members, 1672-1945; royal appointments and honours, 1795-1948; central government papers, 1581-1887; county administration papers, 1518-1904; and administration records of the church, schools and charities, 1598-[1876x1904]. Other component parts of the archive are the Clenennau Letters and Papers, which combine personal correspondence with the civil and military administration of Caernarfonshire from the late sixteenth to late seventeenth centuries. Additional records, comprising Lord Harlech's Game Books (3 volumes), 1882-1933, a journal kept by W. R. Ormsby Gore of the 13th Light Dragoons, May-September 1854, two manuscript catalogues of plays, 1815, and a manuscript catalogue of the library at Porkington, 1809, were acquired in March 2017.
The Brogyntyn (Longueville) group comprises deeds and documents relating to the Brogyntyn estate, 1607-1977, deposited by Longueville Gittins solicitors who provided professional legal services to the estate.

Important mediæval manuscripts and later literary and historical manuscripts, [12 cent, first ½]-[late 19 cent.], reflecting the collecting interests of the Maurice and Owen families of Clenennau and Brogyntyn.
They include an important mid-fifteenth century miscellany of prose and verse in Middle English (Brogyntyn MS II.1); English and Welsh poetry; plays; astrology and prophecies; chronicles of the history of Britain, one of which is a thirteenth century version of Historia Regum Britanniæ of Geoffrey of Monmouth (Brogyntyn MS I.7); a lute book, [c. 1595] (Brogyntyn MS I.27); a copy of the laws of Hywel Dda [1625x1632] (Brogyntyn MS I.12); legal precedents and other papers of legal interest in Latin and English; pedigrees, genealogy and heraldry of North and South Wales families; religious treatises, prayers, devotions and sermons; a seventeenth-century Latin-Welsh dictionary and other manuscripts of linguistic interest; extracts from classical literature; commonplace books; academic notes; copies of significant historical letters and documents; political tracts; moralistic and philosophical works; memoranda, journals and private papers of members of the Anwyl and Owen families; a few Brogyntyn estate and trust papers, 1727-1792; and notes on public offices and official papers deriving from the administration of Oswestry Corporation, 1660, 1673. Some ancilliary materials, [19 cent, second ½]-[1960s], mostly correspondence and notes relating to individual manuscripts, are also included (MSS I.27a, II.1a, II.10a, II.22a, II.42a, II.54(h), II.56a).

A facsimile manuscript in two parts mostly in the hand of William Watkin Edward Wynne. The first part comprises copies (some printed) of charters, public records, deeds, pedigrees, poetry, etc. of Merionethshire and Caernarvonshire interest, some of which are taken from transcripts made by Robert Vaughan, Hengwrt. The material includes records and pedigrees relating to the Wynn family of Peniarth; notes on the Maurice and Owen families of Clenennau, Penmorfa, Caernarvonshire, with related deeds possibly in the hand of William Maurice of Llansilin; deeds relating to the Porkington estate; an extent of the commote of Eifionydd, 1352; an extract from the Coroner's Rolls for Merionethshire, 1345; charters of Castell y Bere and Harlech Castle; pedigrees of Madog ap Dafydd of Hendwr, Llandrillo, Merionethshire; an ode to Einion ap Gruffydd of Corsygedol by Gruffudd Gryg; odes to Dafydd ab Ieuan ab Einion by Guto'r Glyn and Dafydd Nanmor; letters addressed to W. W. E. Wynne, the correspondents including Walter Davies ('Gwallter Mechain'); etc. The second part is also mostly in the hand of W. W. E. Wynne and again comprises material mainly of Merionethshire and Caernarvonshire interest, including pedigrees, correspondence, deeds, etc. relating to the Porkington estate and to the Maurice family and to the Wynne family of Glyn and Ystumcegid, Caernarvonshire; poetry relating to members of the Wynn family of Glyn by Huw Machno, Rhisiart Cynwal and others (one elegy translated into English); press cuttings taken from the Cambrian News, 1879; letters addressed to W. W. E. Wynne, the correspondents including Walter Davies ('Gwallter Mechain') and Joseph Morris; etc.