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Estate and family papers of Owen and Wynne families of Peniarth, Merionethshire, [15 cent.]-[19 cent.], including groups relating to Mostyn of Nant and Mostyn and Williams of Penbedw, Flintshire, to Maurice of Lloran, Denbighshire, and to Corbet of Ynysmaengwyn, Merionethshire, including estate papers, 1630-1870, rentals and accounts; deeds, 1361/2-1963, mainly for Peniarth, Aberllefenni, Penbedw, Drenewydd and Mallwyd estates; legal papers, 1539-1848; industrial papers, 1615-1852; county administration, 1468-1874; and non-family trust papers, 1468-1878, mainly relating to the Ynysymaengwyn estate.

Papers of Sir Henry Haydn Jones comprising letters dealing with local government affairs, education, elections, local industries, agriculture, and other activities, 1899-1950; correspondence relating to a hymn and tune book compiled by him, 1915-1917; miscellaneous papers, 1836-1880, the earlier papers belonging to his father, J. D. Jones; notebooks containing sermon notes; papers relating to Towyn British School, 1858-1862; Ruthin British School visitors' books, 1849-1864; and papers relating to the Maesypandy and Ynysymaengwyn estates, 1858-1883, the Abergynolwyn Slate and Slab Company, 1924-1939, and the Talyllyn Railway, 1924, 1938-1949.