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Deeds and documents relating to the Harpton Court estate in Radnorshire and Breconshire, 1564-1910, but mainly eighteenth and nineteenth centuries, including deeds relating to the Forest of Radnor, 1635-1732, deeds concerning the rectory and tithes of Old Radnor, 1607-1876; cash and account books, 1856-1889, and rent books, 1820-1857; papers relating to the corporation of New Radnor, 1699-1833, produced to a Commission of Enquiry, 1833; papers relating to parliamentary elections, 1741-1910, in Radnorshire, Radnor boroughs, Herefordshire, and Peterborough, including poll books for Radnorshire, 1741, Herefordshire, 1852, and Peterborough, 1852; manorial records for manors in Radnorshire, 1541-1926; and personal papers of various members of the Lewis family including the correspondence of Thomas Lewis, MP, John Lewis, Anne Frankland (later Lewis), Sir Thomas Frankland Lewis, and in particular corespondence and papers of Sir George Cornewall Lewis, including papers relating to Malta, 1830-1855, the Poor Law, 1827-1855, the War Office and India, 1861-1866.

Estate and family records of the Williams family of Penpont, Breconshire, mostly relating to the estate in Breconshire, including deeds, 1314-1871; rentals, 1769-1807; assessments of taxes (window, land, house and horse) in the hundreds of Merthyr and Devynnock, Breconshire, 1743-1787; and letters from members of the Williams family of Penpont, 1793-1828.

Estate and family records of the Gunter family of the Priory, Abergavenny, [c.1545]-^[ITc.1712], and the Milborne family of Wonastow, Monmouthshire,and earlier of Milborne Port, Somerset, comprising deeds relating to properties in Monmouthshire, Breconshire and Herefordshire, [c.1231], 1282-1810, but mainly 1450-1750, records relating to the manors of Wonastow, Grosmont, Skenfrith, and Whitecastle, 1480-1625, accounts, 1698-1765; family correspondence of the Gunter and Milborne families, [c.1621]-[c.1811]; and accounts of Charles Milborne in the Pipe Office, 1699-1730.

Records of the Welsh estates of the dukes of Beaufort, earlier the earls of Worcester and William Herbert, earl of Pembroke (d. 1469), including records for the Breconshire lordships of Crickhowell, from 1382, and Tretower, from 1532; ministers' accounts for Monmouthshire lordships from 1387 and manorial records for the lordship of Chepstow, from 1568, Monmouth, from 1416, Porthgaseg, from 1262, Raglan, from 1364, Treleck, from 1508, and for the lordship of Usk, from 1517; records for the Seignory of Gower and Kilvey from 1366 and for the borough and manor of Swansea, 1657-1835; deeds from the 13th cent.relating to the Badminton estate in Monmouthshire, Breconshire and in Gower, Glamorganshire; records from the 16 cent. relating to the coal and iron industries in Monmouthshire and Glamorgan; and estate management records including rentals, 1638-1933, accounts of rent arrears, 1669-1839, bailiffs, collectors and stewards' accounts, 1652-1858, and registers of leases, 1629-1918.

Records relating chiefly to the Welsh estates of the Wood / Lockwood family, comprising volumes of rentals and disbursements, 1830-1843, and manorial records, 1564-1849; about 550 autograph letters relating to the management of the Wood estates in Monmouthshire and Glamorgan, 1836-1853; over 500 deeds relating to properties in Glamorgan, Monmouthshire, Anglesey, Breconshire, Radnorshire, Surrey and Middlesex, 1640-1891; and documents relating to various industrial activities, 1838-1905.

Records of the Morgan family of Tredegar and Ruperra, later barons and viscounts Tredegar including deeds, 14th-20th cent. of the Tredegar, Ruperra, Dderw and Palleg estates in Monmouthshire, Glamorgan and Breconshire which document much of the growth of the towns of Newport and Cardiff in the 19th century; records of the lordship of Wentlloog (Newport) and many Monmouthshire manors, some 14-16 cent., but mainly 17-19 cent.; records of the manor of Brecon and of other manors in Breconshire, 17-19 cent. including the Great Forest of Brecon; records of industrial interests, mainly coal and iron in Glamorgan and Monmouthshire, 18-20 cent.; records of the Tredegar Wharf Company from 1807; and surveys, audit books, rentals, ledgers and leases for the Monmouthshire, Glamorgan and Breconshire portions of the Tredegar estate, 18-20 cent.; papers relating to Nova Scotia and Canada, 1730-1773, mainly of Richard Phillips, Governor of Nova Scotia, 1717-1749; and rentals and leases for the Mile End and Bow estates in London, 19-20 cent.