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Research papers of Kenneth E. Skinner, 1911-1979, mainly notes, photocopies and manuscript and typescript transcripts of unpublished material collected by Dr Skinner while undertaking research in Britain and Argentina for his doctoral thesis 'The relationship between the Welsh colonies in Chubut and the Argentine government'; printed material and periodicals, 1921-1979; and a photograph album of views of Chubut.

Papers of and acquired by R. Bryn Williams, mainly relating to the Welsh settlement in Patagonia, including a diary of Joseph Seth Jones, one of the first wave of emigrants on the Mimosa to Patagonia, 1865, and correspondence, 1865-1868; correspondence of his brother, Robert Charles Jones, 1867-1877; copy records of the Welsh courts in Y Wladfa, 1872-1881; letters and minute books relating to Vrondeg Baptist Chapel, 1875-1887, Gaiman, 1877-1891, Eglwys Llanddewi, 1891, Eglwys Bryn Gwyn and Cyfarfod Misol Y Wladfa (Calvinistic Methodists), 1881-1955; papers relating to the Centenary Celebrations of the Welsh settlement in Patagonia, 1952-1962; letters from the founders of the Welsh colony, 1866, and from others who had experienced life there; letters to R. Bryn Williams from Patagonia and from Wales relating to Patagonia, [c. 1941-1961]; research notes and manuscripts of books and radio plays by R. Bryn Williams, 1942-1962; miscellaneous records relating to Wales and elsewhere collected by Williams, 1865-1962; papers relating to John S. Williams, 1901-1962; papers and press cuttings on the history, culture and industry of Patagonia, 1869-1962; and typescripts of published and unpublished works, lectures, scripts, etc.