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Papers of Arthur John Williams, 1881-1943, including political papers comprising letters, 1868-1911; papers relating to legal, electoral and land reforms, 1867-1911; papers relating to his parliamentary elections in Birkenhead and Glamorgan, 1880-1895; papers relating to South Glamorgan politics, 1886-1924; material concerning the National Liberal Club, 1883-1951; diaries, 1864-1911; diaries of Rose Harriette Thompson Crawshay 1868-1943; and family and financial papers, 1767-1943.

Papers of D. Caradog Jones, [c.1940]-1978, comprising records relating to the Labour Party and Welsh rural areas, 1951-1959; general correspondence, 1951-1978; and papers and press cuttings, [1940x1959], concerning D. Caradog Jones and Montgomeryshire politics, 1940s-1950s.

Papers of D. Emlyn Thomas, 1936-1954, mainly constituency correspondence, 1946-1954, as Labour Member of Parliament for the Aberdare division of Glamorganshire; and pocket diaries, 1937-1954, containing brief notes of appointments and other comments.

Papers of Gwilym Jones, MP, including constituency files, 1983-1997; questionnaire replies, 1985-1995; and subject files, 1980-1997, relating to local, national and international issues.

Card indexes to the papers previously donated.

Papers collected by John Bryn Roberts, including correspondence, 1830-1887; legal certificates, 1863-1897; diaries, 1838-1930, kept by Bryn Roberts and some other members of the Roberts family; photographs, [c. 1880]-1924; notes on legal cases and topics, [c. 1902]-[c. 1921]; letters, 1888-1926, from John Bryn Roberts to the press; newspaper reports transcribed, 1883-1905; notes for his speeches, 1885-1905; notes on political topics, [c.1892]-[1926]; general notes, [1860]-[1894]; election addresses, 1885-1924; political leaflets and pamphlets, 1880-1927; official publications, 1889-1927; legal publications, 1863-1930; miscellaneous printed matter, 1883-1925; Calvinistic Methodist papers, 1844-1928; papers relating to the University of Wales, mainly the University College of North Wales, Bangor, 1882-1926; newspaper and magazine cuttings, 1874-1929; newspapers and periodicals, 1902-1928; bills and receipts, 1781-1926; notebooks and account books, 1833-1900.

General and parliamentary correspondence, 1961-1987; constituency correspondence, 1970-1987, files relating to constituency affairs, 1947-1987; files relating to the following: Welsh affairs, 1985-1987, including transport, 1959-1973; health service, 1960-1978; Welsh language and nationalism, 1966-1979; devolution, 1970-1979; Select Committee for Welsh Affairs, 1975-1985; the Labour Party, 1964-1987, mainly annual conferences and general elections; industrial affairs, 1958-1985, penal reform, 1961-1987, children, 1968-1987, abortion, 1969-1979, nuclear energy, 1977-1987, genetic engineering, [c. 1977] - 1985; and personal papers, mainly letters, [1930s]-1946, and articles, notes and diaries, [1930s]-[1980s]. A further consignment of papers were received. These remain uncatalogued.

Correspondence and papers relating mainly to Lord Hooson's political career, including papers regarding parliamentary questions, 1967-1978; the Welsh Liberal Party, 1963-1979; Montgomery County Liberal Association 1965-1979; Welsh Affairs, 1961-1978; University College of Wales, Aberystwyth, 1961-1968; Dyfed-Powys Constabulary, 1970-1976; foot and mouth disease in Wales, 1967-1968; transport problems in Mid-Wales, 1962-1974; National Theatre for Wales, 1968-1969; Rural Development Board for Wales, 1967-1970; Mid-Wales Hospital Service, 1972-1973; Farmers Union of Wales, 1966-1973; Aberfan Disaster, 1966-1967; television and radio reception in Wales, 1969-1976; Wales Tourist Board, 1968-1976; Plaid Cymru, Welsh nationalism, Welsh language, Devolution, Federalism, Welsh economy, unemployment, Rhondda West by-election, etc., 1960s-1970s; the Liberal Party correspondence, 1960s-1970s, Liberal Party organisation and policies, 1967-1971; Liberals and the Industrial Relations Bill, 1971-1973; Lib-Lab pact, 1977-1978; Liberal Foreign Affairs Panel, 1966-1967; NATO and the North Atlantic Assembly, 1966-1978; correspondence files of the Welsh Liberal Party, 1966-79; engagement diaries, 1966-1978; typescript speeches and notes for speeches, 1960s-1970s; parliamentary accounts, 1970-1972; miscellaneous speeches, press statements, newspaper cuttings, etc., 1960s-1970s; political papers [c. 1950]-1973, produced by various parties; Local Government Reform in Wales, 1993-1994; the Liberal Party's Pantyfedwen Conferences, 1956-1963; the London Welsh School, 1983-1993, the Llangollen International Eisteddfod, 1986-1997; the provision of speech therapy and physiotherapy in Clwyd, 1984-1990; constituency correspondence and papers, [1960]-1979; personal correspondence, 1965-1979; and correspondence, press releases and newspaper cuttings relating to Jeremy Thorpe, former leader of the Liberal Party, 1967-1979; together with papers relating to his business interests including, Laura Ashley Holdings Plc., 1984-1997; Severn River Crossing Plc, 1990-1997; and his legal career, 1949-1962. A further collection of Lord Hooson's papers were received in May 2011 - this group remains uncatalogued.

Papers of Stuart Rendel and family members, including papers relating to the University College of Wales, Aberystwyth, and the proposal to establish the National Library of Wales and its development during the early years of its existence, 1883-1916; speeches, addresses and political papers relating to disestablishment of the church in Wales and the 1889 Intermediate Education Act, 1882-1909; press cuttings, 1881-1913; photographs, 1892; miscellaneous letters, 1878-1912; letters to Stuart Rendel, 1853-1912, including letters from A. C. Humphreys Owen, 1877-1905, family letters, 1853-1902, and letters from prominent political figures and Welsh public figures; letters and copies of letters from Rendel, 1880-1912; diaries, mainly recording details of Stuart Rendel's business activities, 1863-1869; notes of conversations with W. E. Gladstone, John Morley and H. H. Asquith, 1888-1910; papers relating to Chinese affairs and French and Chinese peace talks, 1884-1886; papers of James Meadows Rendel, including letters, 1828-1856, and papers relating to his estate, 1856-1859; letters of Catherine Jane Rendel, 1845-1855; letters and papers of George Wightwick Rendel, 1871-1902; papers relating to Rendel's other brothers, 1841-1889, and his daughters, 1882-1910; letters and papers of Harry Stuart Goodhart-Rendel, 1898-1959, and other papers concerning him, 1963-1977; papers, mainly letters, of the Goodhart family, 1819-1957; papers of Miss Rosemary Rendel, 1986-1996; papers of Sir George William Rendel, including: Foreign Office papers, 1917-1967, correspondence, 1912-1973, papers relating to the Catholic Union of Great Britain, 1942-1979, lectures, diaries and notes, 1915-1954, personal and family papers, 1908-1980, and material relating to the book The Sword and the Olive (1957), 1954-1986.

Papers of Merfyn Jones relating to the Liberal Party, 1964-1989, comprising papers and correspondence of the National Liberal Association, 1964-1988; papers, correspondence and minutes relating to the Welsh Liberal Party, 1965-1987, and on subjects including policy, 1969-1986, devolution, 1976-1979, and European Elections, 1977-1984; correspondence and minutes relating to Ceredigion and Ceredigion and Pembroke North Liberal Associations, 1966-1988, and papers relating to general and local elections, 1973-1987; papers relating to Aberystwyth Liberal Association, 1968-1988, to University College of Wales, Aberystwyth, 1977-1989, and to the Association of University Teachers, 1979-1988; newspaper cuttings, 1964-1988; personal papers of Merfyn Jones and correspondence with Liberal politicians, 1965-1988; printed material, [1968]-1987; papers relating to Young Liberals at national and local levels, 1966-1976; papers relating to the Social and Liberal Democrats, 1984-1988.

Llythyrau cyffredinol, 1939-2002, wedi eu cyfeirio at Gwynfor Evans, ynghyd â ffeiliau o lythyrau, 1940-1996, oddi wrth bedwar-ar-ddeg o unigolion blaenllaw a fu'n gohebu'n gyson â Gwynfor Evans; ffeiliau ar bynciau penodol, 1968-1983, ynghyd â ffeiliau cyffredinol ar bynciau amrywiol, 1971-1979; a ffeiliau amrywiol, 1929-1981; papurau personol amrywiol, 1938-2001, a phapurau amrywiol, [c. 1930-1998]./General letters, 1939-2002, addressed to Gwynfor Evans, together with files of letters, 1940-1996, from fourteen prominent individuals who corresponded regularly with Gwynfor Evans; files on specific subjects, 1968-1983, together with general files on miscellaneous subjects, 1971-1979; and various files, 1929-1981, miscellaneous personal papers, 1938-2001, and miscellanea, [c. 1930-1998].

Papers, 1918-1954, of Professor Robert Richards comprising papers relating to the Commission on Ancient Monuments in Wales, 1919-1954; notebooks containing historical research notes and notes for lectures, extracts from books and journals, reviews, drafts of monographs and articles by Professor Robert Richards, letters from historians and authors, correspondence and papers, 1941-1954, relating to The Monastic Houses of Wales and the Borders; notebooks on economics and economic history; political papers, including material on the agricultural question, 1919-1923, Welsh Affairs, 1945-1954, parliamentary correspondence, 1934-1953, miscellaneous papers, 1918-1947, and papers concerning temperance and religion, 1924-1949; and papers reflecting Robert Richards's interest in nature, 1923-1944, including a diary for the period 1938-1944.

Addresses, lectures and speeches, notes and other papers, 1900-1922, relating to politics, Welsh nationalism, education, rural housing, disestablishment, army recruiting and Sir Ellis's defeat as Liberal candidate for Anglesey; press cuttings, 1883-1926; biographical material, 1949-1954, including an incomplete typescript of a biography by E. Morgan Humphreys; and political letters from Ellis-Griffith, 1873-1926, and letters to him, 1878-1925.

Papers of Sir Henry Haydn Jones comprising letters dealing with local government affairs, education, elections, local industries, agriculture, and other activities, 1899-1950; correspondence relating to a hymn and tune book compiled by him, 1915-1917; miscellaneous papers, 1836-1880, the earlier papers belonging to his father, J. D. Jones; notebooks containing sermon notes; papers relating to Towyn British School, 1858-1862; Ruthin British School visitors' books, 1849-1864; and papers relating to the Maesypandy and Ynysymaengwyn estates, 1858-1883, the Abergynolwyn Slate and Slab Company, 1924-1939, and the Talyllyn Railway, 1924, 1938-1949.

The collection comprises correspondence, including general correspondence to Sir J. Herbert Lewis, 1886-1933, drafts and copies of correspondence from Sir J. Herbert Lewis, 1887-1933, letters from Sir J. Herbert Lewis to Adelaide, his first wife, 1891-1893, letters from Sir J. Herbert Lewis to Ruth, his second wife, 1902-1933, letters from Sir J. Herbert Lewis to his daughter Kitty, 1915-1925, letters from Lady Lewis to Sir J. Herbert Lewis, 1899-1930, letters to Lady Lewis, 1901-1939, and miscellaneous correspondence, 1890-1920; diaries, 1872-1933; Liberal Party in Wales, 1889-1896; subject files (including correspondence), 1865-1933; press cuttings, 1879-1933; deeds and documents, 1442-1864; miscellaneous papers, 1750-1949; and photographs, c. 1890-1929.

Article by Ruth Lewis - 'Early Memories'; letters between Saunders Lewis and Sir Herbert Lewis and other letters; article by Kitty Idwal Jones - 'Early Memories'; article by Olwen Foreman - ''Wartime and College Memories', deposited by Mrs Olwen Foreman, February 2008.

Papers of Sir Samuel Thomas Evans, comprising correspondence, 1876-1920, including letters relating to D. Lloyd-George, personal matters, such as family matters, UCW Essay Prize and Evans' death, political matters and the Welsh Church Commission; miscellaneous political papers, leaflets, notes etc, [1890]-[1910]; miscellaneous notes, pamphlets, notebooks etc. of a personal nature, 1875-[1919]; speeches and notes, [1900-1918]; papers relating to the Welsh Church disestablishment question, [1893], [1908x1910]; legal cases, 1894, 1910-1918; press cuttings, [1890x1918]; and miscellaneous material, 1881-1916.

General personal and political correspondence, 1936-1997, including letters from the Royal Family, MPs and Government Ministers, such as James Callaghan, Margaret Thatcher and John Major; subject files including the Labour Party, 1951-1979, the National Union of Teachers, 1963-1971, Secretary of State for Wales, 1968-1969, Devolution in Wales, 1970-1973, the Christian Heritage, 1977-1985, Aberfan Disaster Fund Bill, 1978-1979, Cardiff West Constituency Labour Party, 1981-1982, the National Children's Homes, 1981-1993, British housing, 1984-1985, GT's memoirs, 1983-1985, the College of Preceptors, 1982-1987, the House of Lords, 1985-1987, St George's House, Windsor Castle, 1985-1987, education, 1986-1987, European Union, 1990-1997, the Welsh Assembly, 1996-1997, the WDA, 1991-1992, and various medical and charitable foundations, 1982-1997; miscellaneous political and personal papers, 1927-1997, including material concerning the Cardiff City Labour Group; 1927-1958; religious interests, 1960's-1990's; Speaker's engagements and official papers, 1976-1983; general publications, 1950-1987, including The Gospel Witness, 1955-1983; Parliamentary publications, 1961-1986, The House Magazine, 1980-1991; personal papers, [c. 1940s]-[1990s]; political papers, accumulated as MP for Cardiff West, Government Minister and Member of the House of Lords, 1955-1997; and letters, 1983-1997, from Sir Julian Hodge, relating to European union and devolution.

Papers of William George, Criccieth, consisting of his personal and family correspondence, diaries and notes, 1881-1960, and papers relating to his publications and public life (including political, legal, religious and Welsh cultural material), 1883-1958, together with diaries, 1881-1915, of Richard Lloyd ('Uncle Lloyd'), and a considerable amount of correspondence and other papers relating to members of the George family, the Lloyd family and the Lloyd George family, 1766-1981. Of particular interest is a very substantial group of papers of David Lloyd George, including: correspondence with William George, mostly 1886-1918; diaries, 1878-1892; letters from prominent politicians, 1879-1913; other letters, including many to family members, 1883-1928; letters from his secretaries, 1906-1963; and working drafts and notes in preparation for his speeches.