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Manuscripts and rare books relating mostly to the counties of Brecknockshire and Carmarthenshire, on subjects such as history, topography and especially genealogy, 1604-1859, including a transcript of the Golden Grove Book of pedigrees and other pedigrees, relating mainly to South Wales families; 19th century transcripts and copies of letters, including some from Sir Walter Raleigh, [1624]-[1807]; lists of Carmarthenshire sheriffs and Brecknockshire Lords Lieutenant, 1809-1849; parts of original manuscripts of Theophilus Jones and William Owen Pughe, [1792]-[1805]; notebooks and scrapbooks, 1839; and various annotated printed books; and deeds and other documents, 1588-1911, relating mostly to properties in Brecknockshire (particularly in the parish of Bronllys), with a few relating to Carmarthen and Swansea.

Records and court rolls, 1832-1936, mainly relating to the manors of Anhuniog, Creuddyn, Cyfoethbrenin, Mebwynion, Mefenydd, Perfedd, Tal-y-sarn and Silian, in Cardiganshire, 1874-1936, and the manors of Caeo, Catheiniog, Glyncothi and Bwlchcymbyd, Mabelfyw, Mabedrud, Maenordeilo, Mallaen, Pennant Forest and Talley, in Carmarthenshire, 1883-1934; copies of surveys of Talley, 1832; and miscellaneous documents, 1842-1858.

Deeds, 1609-1873, mostly relating to lands in Carmarthenshire, including the Trimsaran estate; records of the Commissioners of the Kidwelly and Llanelli Canal and Tramroad Act, 1813-1834; and deeds and records of the Llanelli Canal and Tramroad Company, 1834-1839. The fonds does not contain any records relating to the Carmarthenshire Antiquarian Society.

Deeds relating mainly to Cardiganshire and Carmarthenshire, 1782-1951, including deeds of the Johnes family of Hafod, Cardiganshire, and rentals of manors in Cardiganshire and Carmarthenshire, [c. 1891]-1925, including the manor of Tal-sarn and Silian, [c. 1891]-1916.

Financial records and correspondence of the Association, 1913-1955; annual reports, 1880-1957; account book and Annual Reports of the Association's Home Mission 1895-1953; and financial and other papers of the Young People's Association, 1948-1953.

Deeds collect by J. Augusta Berry, mainly relating to properties in Glamorgan, Pembrokeshire and Carmarthenshire, 1753-1865.

Deeds and documents relating to the estate of the Brock family in Carmarthenshire, 1843-75, and others, 1774-1900; and other deeds and documents, 1774-1900.