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Reports, 1915, on the subject of the teaching of agriculture in county secondary schools; translations of a portion of Morgan Lloyd ('Morgan Llwyd o Wynedd'): Llyfr y Tri Aderyn submitted for competition at the University College of Wales Celtic Society 'eisteddfod', 1900.

Articles and addresses by David Samuel mainly on Welsh literature, history and education, 1890-1909, and an account of his tour in the United States of America, 1889.

Minutes and other papers relating to 'Cymdeithas Lenyddawl Gymreig Aberystwyth', 1855-1862, the Aberystwyth Harmonic Society, 1864-1865, and the Aberystwyth Penny Readings Society, 1864-1866, together with letters from D. F. Ellis, Sarah Jane Rees ('Cranogwen') and Edward Williams, mainly to Richard Samuel.

Notes and articles by David Samuel on Welsh literature, including addresses entitled 'Theophilus Evans a Drych y Prif Oesoedd' and 'Some local ballad singers and ballad writers'.

Papers, 1816-1930, of David Samuel (Dewi o Geredigion), including material mainly of Aberystwyth interest; correspondence; lectures and articles; examination papers in Welsh grammar, literature and history; and miscellaneous notes.

Notes on Welsh grammar, idioms, loan words and dialect words, the teaching of Welsh in schools, etc. by David Samuel, D. Tecwyn Evans, Sir John Morris-Jones, T. Gwynn Jones, Sir John Rhys, etc.

Notes on Welsh grammar, idioms, loan words and dialect words, the teaching of Welsh in schools, etc. by David Samuel, D. Tecwyn Evans, Sir John Morris-Jones, T. Gwynn Jones, Sir John Rhys, etc.

Notes on Welsh grammar, idioms, loan words and dialect words, the teaching of Welsh in schools, etc. by David Samuel, D. Tecwyn Evans, Sir John Morris-Jones, T. Gwynn Jones, Sir John Rhys, etc.

Scriptural notes, addresses, examination questions, sermons and notes of sermons, papers relating to the Calvinistic Methodist connection, mainly in Aberystwyth and district, etc.

Lectures, articles and notes by David Samuel on the history of Aberystwyth and neighbourhood.

Letters to David Samuel from R[ichard] Trevor Owen, Edward Owen, Rupert H[ugh] Morris, W[illiam] Basil Jones (bishop of St Davids), J[ohn] Mortimer Angus, John Lewis ('Ap Cletwr'), Joseph Brough, H[enry] Tobit Evans, John Owen (afterwards bishop of St Davids), David Jenkins (Llangwyryfon), Arthur Johnson Hughes, L[ewis] J[ones] Roberts, etc. relating to the visit of the Cambrian Archaeological Association to Aberystwyth in September 1896, together with minutes of the Aberystwyth local committee.

Letters, 1889-1902, from D. Silvan Evans to David Samuel.

A history of Salem Calvinistic Methodist Church, Aberystwyth compiled by David Samuel, together with related press cuttings, 1893-1921.

A sales book, 1816-1840, kept by Samuel Williams and his successors, printers, booksellers and stationers, Aberystwyth.

Examination papers on Welsh grammar, literature and history set by 'Gorsedd Beirdd Ynys Prydain', the University of Wales, St David's College, Lampeter and the Central Welsh Board for Intermediate Education, 1912-1916.

Notes on scriptural and theological subjects and outlines of sermons preached at Aberystwyth by Calvinistic Methodist ministers.

Articles and notes by David Samuel on Llandovery School, Sir Owen M. Edwards and D. Silvan Evans.

A notebook used by David Samuel containing quotations from the English poets, notes made during a tour in North America and a diary kept by him, 1900-1901.

Minutes, letters and other papers relating to the reading circles arranged by the Free Church Council in Aberystwyth, 1905-1909.

Miscellanea of David Samuel, including articles, notes on the centenary of the introduction of the printing press to Aberystwyth and other notes of local interest, an appreciation of Sir Owen M. Edwards, etc., together with an account of the formation of a branch of 'Undeb y Ddraig Goch' at Aberystwyth, 1902.