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A short biographical sketch of David Samuel transcribed by him from Columbia (1890), a Welsh newspaper published at Emporia, Kansas, U.S.A., and a list, also by David Samuel, of articles contributed by him to various periodicals, 1884-1920.

Press cuttings and notes relating to the Aberystwyth County School and the activities and successes of its pupils.

Letters, 1879-1920, to David Samuel from Sir Edward Anwyl, J[ames] F[ranklin] Bethune-Baker, D[avid] H[enry] Davies (Cenarth), Sir Owen M[organ] Edwards, Thomas Edwards ('Gwynedd'), D[avid] Tecwyn Evans, Gruffydd Evans (Newcastle Emlyn), John Young Evans, S[amuel] J[ames] Evans (Llangefni), C[harles] L[ett] Feltoe, E[dmund] Tyrrell-Green, [James] Rendel Harris, David Howell ('Llawdden'), J[ames] Spinther James ('Spinther'), Edward Jenkins (Llandrindod Wells), Evan Jones (Caernarvon), Gwilym Hywel Jones, J[ohn] Cynddylan Jones, John Morgan Jones (Cardiff), Sir John Morris-Jones, T[homas] Gwynn Jones, T. Wolseley Lewis, Thomas Lloyd (Liverpool), William Morgan (Pant, Dowlais), Sir Hugh Owen, O[wen] G[riffith] Owen ('Alafon'), E. Wynne Parry (Bala), T[homas] Mordaf Pierce, Thomas Powel, Evan Rees ('Dyfed'), Sir John Rhys, Eleazar Roberts, L[ewis] J[ones] Roberts, Robert Arthur Williams ('Berw'), W[illiam] Gilbert Williams, etc.

Copies of articles by David Samuel printed in Y Cymro, Y Brython, Y Cerddor, etc., 1913-1930.

Miscellaneous short articles and notes, including notes on Welsh funeral customs, mainly by David Samuel, press cuttings, etc., 1888-1896.

Articles, addresses, notes and press cuttings by David Samuel relating to Aberystwyth, D. Silvan Evans, etc., 1887-1895.

Articles, notes and addresses by David Samuel.

Miscellanea of David Samuel, including articles, notes on the centenary of the introduction of the printing press to Aberystwyth and other notes of local interest, an appreciation of Sir Owen M. Edwards, etc., together with an account of the formation of a branch of 'Undeb y Ddraig Goch' at Aberystwyth, 1902.

Minutes, letters and other papers relating to the reading circles arranged by the Free Church Council in Aberystwyth, 1905-1909.

A notebook used by David Samuel containing quotations from the English poets, notes made during a tour in North America and a diary kept by him, 1900-1901.

Notes on scriptural and theological subjects and outlines of sermons preached at Aberystwyth by Calvinistic Methodist ministers.

Articles and notes by David Samuel on Llandovery School, Sir Owen M. Edwards and D. Silvan Evans.

Examination papers on Welsh grammar, literature and history set by 'Gorsedd Beirdd Ynys Prydain', the University of Wales, St David's College, Lampeter and the Central Welsh Board for Intermediate Education, 1912-1916.

A sales book, 1816-1840, kept by Samuel Williams and his successors, printers, booksellers and stationers, Aberystwyth.

A history of Salem Calvinistic Methodist Church, Aberystwyth compiled by David Samuel, together with related press cuttings, 1893-1921.

Letters, 1889-1902, from D. Silvan Evans to David Samuel.

Letters to David Samuel from R[ichard] Trevor Owen, Edward Owen, Rupert H[ugh] Morris, W[illiam] Basil Jones (bishop of St Davids), J[ohn] Mortimer Angus, John Lewis ('Ap Cletwr'), Joseph Brough, H[enry] Tobit Evans, John Owen (afterwards bishop of St Davids), David Jenkins (Llangwyryfon), Arthur Johnson Hughes, L[ewis] J[ones] Roberts, etc. relating to the visit of the Cambrian Archaeological Association to Aberystwyth in September 1896, together with minutes of the Aberystwyth local committee.

Lectures, articles and notes by David Samuel on the history of Aberystwyth and neighbourhood.

Scriptural notes, addresses, examination questions, sermons and notes of sermons, papers relating to the Calvinistic Methodist connection, mainly in Aberystwyth and district, etc.

Notes on Welsh grammar, idioms, loan words and dialect words, the teaching of Welsh in schools, etc. by David Samuel, D. Tecwyn Evans, Sir John Morris-Jones, T. Gwynn Jones, Sir John Rhys, etc.