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A collection, entitled 'Y Brasnadd Newydd Medi'r 22nd. 1817', of a hundred and sixty four hymns based on the Psalms and other portions of Scripture by Edward Williams (Iolo Morganwg), similar to those included in his Salmau yr Eglwys yn yr Anialwch, 1812 and 1834. Some of the hymns are accompanied by tunes.

A collection of psalm-tunes ('erddiganau salmau') by Edward Williams (Iolo Morganwg).

A collection of eighty-six hymns entitled 'Salmau. Casgliad Trefflemin. 1824', by Edward Williams (Iolo Morganwg).

A copy of Dagrau yr Awen neu Farwnad Lewis Hopcin Fardd, o Landyfodwg, Iorwerth Gwilim o Dre-fflemin ym Morganwg [i.e. Iolo Morganwg] a'i Cant (Pony-y-fon: R. Tomas, 1772), with some manuscript emendations by the author.

A pocket-book which belonged to 'Edwd William Junr' [i.e Iolo Morganwg] containing entries made [c. 1767]-[?1775] (undated after 1771). The entries consist of accounts in connection with work done, etc., 'englynion', 'cywyddau' (incomplete), some English verse, lists of words taken mainly from the poems of Dafydd ap Gwilym, a few proverbs, and various memoranda including the following: 'My Dear Mother Died ye 19th day of august 1770 about half an hour past one in ye= morning'. Another note lists various items 'Reced of Mr Waters [sic]', the first two being '1numbr of ye Dictionary' (2s.) and 'ode to humanity' (6d.). Most of the 'englynion' are by EW himself, but a few are by William Robert and one or two other poets. One series (englynion by certain 17th cent. poets) may be found, with minor differences, at the beginning of John Prideaux, Euchologia; nev, Yr Athrawiaeth i arfeol Weddio... Cyfieithiad Row. Vaughan Esc. Ar Ddeisyfiad William Salesbury Esc... ([London]: E. C[otes] tros P. C[hetwin], [c. 1658], ESTC R182098). EW, who styles himself variously as 'Iorwerth ab Iorwerth' and 'Iorwerth Gwilym', has some 'englynion' addressed to 'Lewis Hopcin', 'Ieuan fardd Du', and 'Dafydd meredydd argraffydd or bontfaen', etc. The references to the poems of Dafydd ap Gwilym correspond to some extent to the numbering of the poems in the latter part of Llanover MS C3 [now NLW MS 13090E]. Other references correspond to page numbers in Edward Lhuyd's Archaeologia Britannica (1707). The handwriting varies considerably, and shows a distinct change after c. 1771.

'Some Account of an Ancient Welsh Colony, And their Descendants at present existing, In the interior parts of North-America. by Edward Williams...'. Inside the front cover is 'A Sketch of the Country of the Madogwys 1792' by William Owen. At the reverse end is a note written by (Capt.) Wm Jones, thanking his friend Edwd Williams for the perusal of this manuscript; 'hopes to hear more Authenticated accounts in the Course of this ensuing Year - would also be glad at any time of a line when convinient respecting plans in agitation'. His address.

Letters on Universal Legislation: Letter 1st - Introductory; Letter 2d - Commerce; Letter 3d - Fashion; Letter 4th - Great Cities; Letter 5th - Constitution. Written by Iolo Morganwg: the first letter is dated London, Octr 20th 1792. Incomplete.

A copy of The Daily Journal for 1780, with some manuscript entries by Iolo Morganwg.

(a) A copy of a diary or journal for 1786, with manuscript entries (including English and Welsh verse, etc.) by Iolo Morganwg. At the beginning is 'A Song in praise of Glamorgan' attributed to Sir John Stradling of St Donats; 'From a MS of the late Wm Roberts of Lancarvan, who told me that he had it from one Mr Bassett of Bonvilston, Grandfather of the present Mr Bassett'. (b) Part of another diary, year not given.

'Castles in the Air, By a Journey-man Mason', being a collection of English verse by Iolo Morganwg, in two volumes. The poems are not in their final form, and alternatives are often given above or below the original words. The pages in the first volume are numbered 1-140; the second volume is a continuation to p. 191, followed by 59 unnumbered pages. The first volume contains an index as far as p. 169.

Three small notebooks marked 'Miscellanies', 'Lyric Pastorals', and 'Songs' respectively. The contents include early versions of some of the poems printed in Poems Lyric and Pastoral (1794).

An imperfect collection of English poems by Iolo Morganwg, with an index to the contents. The entire collection contained 55 or more pages, and those preserved here are numbered 7-22, ?27-28, 33-40, and 43-48. The contents include early versions of some of the poems printed in Poems Lyric and Pastoral (1794).

'Poems on several occasions, By Edward Williams, A Journeyman Mason'. There are 39 items in the list of contents at the beginning, and many of the poems are to be found in Poems Lyric and Pastoral (1794), but with considerable differences. The cover consists of two leaves from John Walters' Dictionary, Citatory - Clean.

'Proposals for printing by Subscription. Poems, Lyric and Pastoral. By Edward Williams, a self-tutored Journey-man Mason, of the County of Glamorgan, in Wales ...', followed by a few of the poems printed in Poems Lyric and Pastoral (1794), Vol. I.

Fragments of collections of English poems by Iolo Morganwg, comprising early versions of Poems Lyric and Pastoral and other poems not included in the printed volumes. Above some of them Iolo Morganwg has written such comments as 'In New Collection much altered' or 'Copied for press', and in one instance 'Copied 1803, for addenda'.

Eight songs or poems mainly of a political nature, several of which are marked 'Copied 1803' (Probably copied into No. 47 [i.e. NLW MS 21335B).

'Proposals for printing by subscription a new and improved edition, with aditions [sic], of Poems Lyric and Pastoral By Edward Williams,' followed by seventeen poems, including a few shorter items (epitaphs).

The manuscript of Salmau yr Eglwys yn yr Anialwch, Cyfrol I (Merthyr Tydfil, 1812). The printed volume contains 204 hymns: the last in the manuscript collection is numbered CC. The preface appears to correspond to the printed copy except that the last paragraph but one is wanting here: there is also another draft of a preface dated 'Trefflemin, neu fal ai gelwid gynt Llanfihangel y Twyn, gerllaw'r Bont faen ym Morganwg Alban Hefin 1811' (found elsewhere among the papers). The index which appears to be a draft is to the printed volume and not to the manuscript.

'Salmau yr Eglwys yn yr Anialwch (Cyfrol II)...'. In the note, dated 7 August 1826, in NLW MS 21339A Iolo Morganwg refers to this volume thus: 'Gweler ym mhrifddarpar yr ail gyfrol 74' [i.e. Salmau]. The collection is similar to, but not identical with, the first pages of the second volume published by Taliesin Williams in 1834: there are some hymns in the MS which are not in the printed volume, and vice versa. There is also a draft of the beginning of a preface (to be found elsewhere).

A notebook designated 'Y Melin Brith', containing Unitarian Doxologies by Iolo Morganwg, some Unitarian hymns, and Byron's Hebrew or Jewish hymns, etc. The pages are numbered 1-32 and there is an outline of the contents on the cover. There is also another copy of the Byron hymns, with music and some notes on 'Jewish Sacrifices, and Ritual', etc.