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Papers, lecture and research notes of and acquired by Mary Williams, relating to Middle French, Middle Welsh and medieval literature and Arthurian studies, 1907-1963; books collected by Mary Williams, 1897-1911; letters to Prof. Victor Spiers, 1898-1916; vouchers and receipts, 1924-1973; newspaper cuttings, 1911-1940; school books 1909-1916; papers relating to University College Swansea, 1921-1975, University of Wales Aberystwyth, 1924-1974, University of Durham, 1948-1952, and National Library of Wales, 1941-1974; correspondence, 1927-1976; and family papers, 1898-1944.

Miscellaneous deeds and documents, mainly relating to properties in co. Card., 1675-1902, co. Caern, 1546-1860, co. Carm., 1702-1914, co. Denb., 1575-1850, co. Flint, 1770-1776, co. Glam., [13 cent.?]-1924, co. Mer., 1598-1890, co. Mont., 1465-1877, co. Mon., 1630-1775, co. Pemb., 1753-1930, co. Rad., 1706-1840, Cheshire, 1703-1789, Gloucestershire, 1656-1788, Herefordshire, 1594-1772, Shropshire, 1710-1809, and Ireland, 1671-1922.

Papers of Alderman R. J. Ellis relating to Aberystwyth Borough Council and Cardiganshire County Council, mainly concerning planning and water, 1937-1975; letters relating to administration of estates, 1902-1976; personal papers, certificates, and diaries of R. J. Ellis, 1910-1972; and a letter from Irish politician Tim Healy, 1886.

Papers of Richard Emrys Bonsall, mainly architectural papers relating to buildings in the Aberystwyth area, Cardiganshire, 1930-1964, including notebook with architectural notes, [c. 1930]-1935; diary of Hywel Owen Jones, 1930-1933; contract certificate counterfoils, 1938-1963; building specifications, 1946-1964; papers relating to alterations to the Wynnstay Arms Hotel, Oswestry and the Royal Hotel, Llangollen, 1955-1964; and copy letters from him, 1959-1961.

Research papers and family history of Theodore White, 1935-1975, comprising theses on chemical and biochemical subjects, submitted to the University of Wales, Aberystwyth, 1935-1939; reports on the industrial extraction of wood products in India, 1964-1968, and on the Quebracho (tanning product) industry, 1971-1975; offprints of articles from scientific journals; and a copy of the donor's family history, which partly relates to the Rhondda, home of his maternal ancestors, in the late nineteenth and early twentieth centuries.

Manuscripts and papers of the families of Charles and Edwards, dated between [c. 1600] and 1922; they include letters from Thomas Charles Edwards to his wife, and their son Lewis Charles, 1876-1896; letters to Thomas Charles Edwards, 1885-1899; copies of letters, 1859-1898, including correspondence relating to University College of Wales, Aberystwyth; letters to and from Mary Roberts, 1867-[1893]; letters to their daughter, Elizabeth Alicia Edwards, 1887-1900; Edwards family letters, 1895-1900; and newspapers and press cuttings, [c. 1820]-1922.

Papers, 1681, 1759-2015, of T. I. Ellis, his wife Mari Ellis and their respective families.
The T. I. Ellis papers consist of correspondence, 1904-1970; personal papers, 1894-1970, including his diaries, 1943-1970; papers relating to his education and career, 1900-1947; financial papers, 1926-1967; papers relating to organisations including Aberystwyth Old Students' Association, the BBC, the Guild of Graduates of the University of Wales, the University of Wales and the Welsh Schoolboys Camp Movement, 1920-1979; papers of committees and commissions with which he was involved, 1932-1968; papers relating to ecclesiastical affairs, the Church in Wales and related bodies, 1909-1991; and correspondence, drafts and notes relating to his publications, 1877-1978.
The Mari Ellis papers, 1681, 1759-2015, include correspondence; diaries, 1930-2014; papers relating to her work in journalism and broadcasting, 1948-2004; and research papers, [?early 20 cent.]-[2008x2010].
Also included are papers relating to the Charles family of Carmarthen and the Davies family of Aberystwyth and Cwrtmawr, 1791-1920; and papers and correspondence relating to T. E. Ellis, 1870-1963, Mrs Annie J. Ellis (later Hughes-Griffiths), 1873-1942, the Rev. Peter Hughes-Griffiths, 1871-1940, J. H. Davies, 1883-1929, and the Headley family, [1890x1896]-[2000s].

Stray papers of the Waddingham family, some of which relate to the Hafod estate, Cardiganshire, 1794-1910, including transcriptions, 1794, of notes on lead mines by Lewis Morris; cost and contract books of Bwlchyranos and South Hafod Lead Mines, 1859-1868; printed Cardiganshire election registers, 1862-1865; miscellaneous press cuttings collected by T. J. Waddingham; estate administration records, including agreements to sell timber for shipbuilding from the Hafod Estate by William Chambers, 1857 and papers relating to water supply and railways; return of copies of a crown land survey adjacent to Hafod, 1845; and various printed pamphlets.

Papers relating to fringe Nationalist and left wing groups, 1963-1989, including material relating to Welsh Nationalist and Republican Groups, 1963-1989, material relating to Welsh left wing groups, 1969-1979, and papers relating to solidarity groups and campaigns, 1968-1989; published political material such as newspapers and periodicals, 1913-1989, records and papers of Cofiwn, 1970-1990, including material relating to the American Indian Movement Tour of Wales, 1986; papers relating to campaigns and activities of groups such as the the Owain Glyndwr Society, 1975-1990; papers relating to maritime history and heritage, 1973-1995; and miscellaneous papers, mainly relating to organisations in Aberystwyth, 1976-1989.

Papers of the UMCA, 1978-1994, including membership files, 1979-1986; accounts, 1981-1994; papers of UMCA officers, 1985-1990; and political correspondence, 1978-1987.

Papurau Aelwyd yr Urdd, Aberystwyth, 1928-1991: cofnodion y cyfarfod cyffredinol blynyddol, y pwyllgor cyffredinol a phwyllgorau eraill, 1928-1990; cofnodion, gohebiaeth a phapurau eraill,1968-1991; a chyfrol o dorion o'r wasg a rhaglenni, 1954-1964 = Papers of Aelwyd yr Urdd, Aberystwyth, 1928-1991: minutes of the annual general meeting, general committee and other committees, 1928-1989; membership books of officials and committee members, 1933-1990; minutes, correspondence and other papers, 1968-1991; and volume of newspaper cuttings and programmes, 1954-1964.

Notes on cataloguing and classification, 1925-1928; correspondence, 1928-1942, 1957; copies of articles and offprints, and cuttings of press reviews; and papers of his father-in-law, Hugh Evans, 1952-1955, mainly notes on publishing, periodicals, etc.

General correspondence files, chiefly financial in nature, with various companies, related bodies such as National Association of Agricultural Services, etc., 1955-1979, correspondence with Ministry of Agriculture and Fisheries, 1930-1957; Ministry of Agriculture, Fisheries and Food, 1957-1968; Agricultural Research Council, 1951-1979; National Institute for Agricultural Botany, 1954-1985; WPBS reports, 1919-1980; annual reports, 1944-196; papers of the Directors and heads of sections, 1919-1974; minutes, etc., relating to various seed production committees, 1947-1957; the papers of Gwilym Evans, 1928-1961; the Cahn Hill Improvement Station at Pwllpeiran, Cwmystwyth, 1933-1973; files of experiments, with details of experiments in progress, field record cards, slips and notebooks, agrotype experiment data, including results of research undertaken at Bicton, Cambridge, Newcastle, Hurley and Aberdeen, and at Welsh county trials, [1919]-1969.

A letter, [Summer of 1923 or 1924], signed 'Tristan', from D. James Jones (Gwenallt), Aberystwyth, to Esyllt Jones (later Mrs Esyllt Clarke, New Zealand), concerning personal matters and describing his day-to-day life in Aberystwyth during the Summer (ff. 190-191).
Also included is an explanatory letter, 24 November 1977, from the donor (ff. 192-193).

Articles, addresses, notes and press cuttings by David Samuel relating to Aberystwyth, D. Silvan Evans, etc., 1887-1895.

Miscellanea of David Samuel, including articles, notes on the centenary of the introduction of the printing press to Aberystwyth and other notes of local interest, an appreciation of Sir Owen M. Edwards, etc., together with an account of the formation of a branch of 'Undeb y Ddraig Goch' at Aberystwyth, 1902.

An album containing press cuttings, reprints of articles in the Aberystwyth Observer, 1899-1905, posters, etc., mainly relating to Aberystwyth and Cardiganshire, and minutes of the committee of the 'Highgate Men's Club', Whitchurch, Shropshire, founded in 1889, with correspondence and other papers relating to the club.

Press cuttings, mainly of Cardiganshire, particularly Aberystwyth, interest, accumulated by members of the Davies family of Antaron, Aberystwyth; two letters from Edward Richard [1714-1777], founder of Ystradmeurig School; posters, broadsides, etc., including a copy of 'Can I. Clod i Ystradmeurig' and 'Can II. Clod i Bont Rhydfendigaid' by J. Hughes, Llwyn-glâs.

An account book, 1877-1891, kept by William Jenkins, bookseller and stationer, Aberystwyth.

An essay on 'Romantic Incidents and Remarkable Characters of Old Aberystwyth' by Evan Lewis, edited for publication by W. R. Hall.