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A collection of manuscripts which includes a copy of Lewis Morris (ed. D. Silvan Evans): Celtic Remains ..., 1878; original poetry and translations; transcripts from various sources, including hymn tunes, anthems, etc., manuscripts, poetry and printed works; correspondence; genealogy; sermon notes; diaries, 1858-1862, 1864, 1871, 1875-1898, and those of Thomas Jones, Owen Jones's father, 1873-1885.

An interleaved copy, with numerous additions and corrections by Owen Jones, of Lewis Morris (ed. D. Silvan Evans): Celtic Remains ... (London, 1878).

A transcript by Owen Jones of William Salesbury: Kynniver llith a Ban or yscrythur lan ac a ddarlleir yr Eccleis pryd Commun y Sulieu a'r Gwilieu trwy'r vlwyddyn ... (London, 1551).

Hymn tunes, anthems, chants, etc. transcribed by Owen Jones, with Welsh and English words added in most cases.

An alphabetical index of place names, mainly in Herefordshire.

Miscellaneous papers, including a letter from Henry Rees, Calvinistic Methodist minister, Shrewsbury to John Jones, Llanfyllin and a genealogical table showing some of the descendants of Thomas Charles, Bala and Sarah Jones, his wife.

Notes of sermons preached, 1828-1829, by John Breese, Dafydd Owen, Evan Davies (Llanrwst), Da[vid] Jones (Treffynnon), William Williams (Wern), John Griffith (Manchester), David Morgan (Machynlleth), John Roberts (Llanbrynmair), Da[vid] Roberts (Dinbych), etc.

A transcript of Jerem[y] Owen: Golwg ar y beiau Y sydd yn yr Hanes a Brintiwyd ... ym mherthynas i'r Rhwygiad A wnaethbwyd yn Eglwys Henllan Yn y Blynyddoedd 1707, 1708, 1709 ... (Caerfyrddin, 1732-1733).

Letters, 1896, from John D. Evans, Talley, Llandilo to Thomas Levi and from E. Wynne Parry, Bala and Richard Jones, Oswestry to Owen Jones relating to Welsh hymns and hymn-writers; transcripts of hymns by Morgan Rhys and William Williams, Pantycelyn and of a portion of Daniel Williams: Gwagedd Mebyd a Ieuengctid ... At yr hyn y chwanegir, Catechism i rai ieuaingc (Llundain, 1739); etc.

A notebook containing lists of books (?bought by Owen Jones) with a record of prices asked or paid for them, together with notes on Greek words, etc.

Miscellaneous letters and papers relating to the affairs of Thomas Jones, father of Owen Jones, together with medical recipes, etc.

The diary of Thomas Jones, father of Owen Jones for the years 1873-1885.

A transcript by Owen Jones of a poem entitled 'Rhybudd y Clwyfus' by Edward Roberts, Capel Garmon and of the last fifteen stanzas of another poem of fifty-seven stanzas contained in NLW MS 527A.

A Hebrew-English vocabulary, scriptural notes and a copy of replies by Thomas Charles Edwards to queries raised by W. O. Jones relating to points of Christian doctrine.

Original poetry and translations by Owen Jones.

A transcript of three translations of Tennyson's 'Guinevere' and of a translation of his 'Sir Lancelot and Queen Guinevere' submitted for competition at the Bangor National Eisteddfod, 1874, together with a short adjudication by Owen Jones.

Notes of lectures on the philosophy of the mind taken by Owen Jones when he was a student at University College, London, 1861.

A transcript by Owen Jones from the manuscript copy in NLW MS 527B of Carwr y Cymru yn annog ei genedl anwyl a'i gydwladwyr ... i chwilio yr Scrythyrau ... (London, 1631).

A collection of proverbs, colloquialisms, allegorical expressions and riddles, including extracts from the works of a number of poets.

Notes by Owen Jones, mainly on elementary science and mathematics.