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A collection of manuscripts, [12 cent.]-1909, from the library of Peniarth, Merionethshire, the core of the historic collection being that of the library accumulated at Hengwrt, Merionethshire, by Robert Vaughan during the seventeenth century. The collection includes many of the most important Welsh language manuscripts, including the Black Book of Carmarthen (Peniarth MS 1), the Book of Taliesin (Peniarth MS 2), the White Book of Rhydderch (Peniarth MSS 4-5) and Brut y Tywysogion (the Chronicle of the Princes) (Peniarth MS 20), as well as important manuscripts in other languages such as the Hengwrt Chaucer (Peniarth MS 392), the Law of Hywel Dda (Peniarth MS 28), Beunans Meriasek (Peniarth MS 105) and Bede's De natura rerum (Peniarth MS 540B).

Papers, 1634-1928, mostly deriving from and relating to the legal practice of Henry Rumsey Williams, comprising draft conveyances, abstracts of title, letters, accounts and miscellaneous papers of clients, including the estate of Wynn of Glynllifon, 1719-1840, the Griffiths family of Caernarfon and Amwlch, 1726-[1830s], Jared Jackson, 1760-1836, Plasgwyn estate, 1761-1846, Cefn Cwmwd estate, 1763-1828, Coed Helen estate, 1770-1838, Trergo estate, 1771-1832, Parry family, 1773-1788, Peniarth estate, 1773-1830, Orielton estate, 1774-1814, Bodior estate, 1778-1837, Faenol estate, 1778-1840, Arnold Robinson Burrowes, 1785-1837, Grindley family, [c. 1786]-1842, Morgan family, 1787-1839, Treiorwerth estate, 1787-1844, Evan Pritchard, 1788-1813, John Price, 1790-1844 Caerhun estate, 1791-1834, W. A. Madocks, 1799-1824, Nancall estate, 1802-1837, Morris Griffith, 1804-1832, Edward Griffith Roberts, 1805-1827, William Humphrey, 1805-1833, Plas Llanfair estate, 1805-1837, Baily Williams family, 1806-1838, Richard Garnons, 1809-1837, Cefn Hengwrt estate, 1810-1815, George Bettiss, 1810-1831, William Edwards, 1811-1836, Penrhyn estate, 1811-1837, Wyatt family, 1813-1835, Gelli Goch estate, 1815-1831, Anna Maria Wynne, 1816-1833, Robert Thomas, 1818-1839, Roberts family, 1818-1840, Bodegroes estate, 1819-1836, Hughes, Brydges and Granville, bankers, 1819-1840, Vickers family, 1820-1833, Boston estate, 1820-1839, Owen Griffith, 1822-1846, George Holmes Jackson, 1823-1841, the Rev. Hugh Hughes Wynne, 1831-1848, John Rowlands, 1832-1841, and Edward Hosier Williams, 1833, in Caernarfonshire, Anglesey, Denbighshire, and Merionethshire; legal correspondence, 1790-1848, probate records, 1727-1871, and papers relating to civil cases, 1757-1850, religion, 1788-1842, mining, 1779-1842, quarrying, 1798-1840, shipping, 1778- [c. 1841], roads and railways, 1834-1839; legal practice records, 1804-1841, and executorship papers, 1841-1855, belonging to Henry Rumsey Williams, and records of his family in Brecknockshire, Monmouthshire and Caernarfonshire, 1881-1928. Records relating to William's political activities have not survived.

A scrapbook, 1867-1882, begun by Evelyn Phillip Shirley of Ettington Park, Warwickshire, following his visit in August 1867 to his friend W. W. E. Wynne of Peniarth, Merioneth.
The volume initially contained ten photographs of Peniarth and its environs (ff. 11, 19, 21, 23, 25, 29, 31, 33, 37, 40) with numerous further photographs (and photographs of prints) being added showing other local views and related houses such as Glyn (ff. i verso-47 passim). Also included are leaves from W. W. E. Wynne's Pedigree of the Family of Wynne of Peniarth… (London, 1872), with hand-painted coats of arms added (ff. 2 recto-verso, 12 recto-verso, 20 recto-verso, 22 recto-verso, 24 recto-verso, 26 recto-verso), and additional manuscript notes by Wynne (ff. 13-18); four letters to Shirley from W. W. E. Wynne, [1868]-1877 (ff. i verso, 3-10, 34-35); three letters, June-July 1880, from W. R. M. Wynne (ff. 41-44) and E[dward] Breese (ff. 45-46), following W. W. E. Wynne's death, with copies of Breese's obituary of Wynne (ff. 50-52); and papers relating to the building and consecration of the Wynne Memorial Church at Bryncrug, 1880-1882 (ff. 53-59).

A group of letters, largely relating to genealogy, heraldry, etc., which include: from Richard Llwyd ('Bard of Snowdon') to Sir William Betham, Herald's College, Dublin, 1814; Robert Roberts, Holyhead to Sir Joshua Meredyth, Dublin, 1814; and W. W. E. Wynne of Peniarth to an unnamed recipient, 1828. The pedigrees mentioned include those of the Powell family of Stanage Park, Radnorshire and of W. W. E. Wynne, Peniarth.

Some forty-eight letters, some incomplete, 1920-1925, to D. C. Lloyd-Owen from Richard Bennett, Bangor and Caersws, concerning mostly Montgomeryshire genealogy (ff. 1-91), together with related genealogical papers (ff. 92-150).
The papers include a list of wills and administrations for 1703-1710 from the Deaneries of Estimaner [and Tal-y-bont], Merionethshire (ff. 92-94); typescript and manuscript extracts from, and notes on, Montgomeryshire wills, 1570-1730 (ff. 95-115, 118-125, 136-138), and Merionethshire wills, 1746-1756 (ff. 148-150); manuscript extracts from Chancery proceedings, (temp. Elizabeth I) (ff. 133-135); and a list of Montgomeryshire wills proved in the Prerogative Court of Canterbury, 1680-1708 (ff. 139-142). The letters include references to notable Montgomeryshire families (ff. 1-6, 9-11, 23, 33, 43, 46, 55-58, 66-69, 129-131) and to the Peniarth (ff. 18, 25, 39, 81, 83, 127-128), Rhiwgriafol (f. 79) and Cwmcarnedd (f. 87) deeds.