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'Collectanea', printed and manuscript, relating mainly to Glamorgan, including copies of charters, copies of an Act of Parliament, dated 31 Henry VIII and printed by Thomas Berthelet in 1544, 'auctorisying the Kynges highnes newely to allotte certayne towneshipes in Wales', memoranda and notes by L. W. Dillwyn, John Montgomery Traherne, and Edward Williams ('Iolo Morganwg'), autograph letters, 1906-1907, from John Stuart Corbett to Sir Thomas Mansel Franklen, etc.

Notebooks used by John Montgomery Traherne to record notes and 'collectanea' mainly relating to the history and topography of Glamorgan, Glamorgan families and pedigrees, and miscellanea. NLW MS 6534A contains notes relating to the Scudamore family.

Posters, broadsides, circular letters, press cuttings, squibs and poems dealing with various Glamorgan parliamentary elections, 1767-1832.

Copies of In the House of Lords. Case of Charles Kemeys Kemeys Tynte, ... Esquire, on his Claim to the Title and Dignity of Baron Wharton of Wharton ... 1843, the report of the Wharton peerage case extracted from Clark and Finelly's Cases in the House of Lords ..., 1845, and other relevant material.

Pedigrees of Glamorgan and other South Wales families, including those of Turberville, Gamage, Stradling, Bassett, Maunsell, Fleming, Button and Kemys, 'supposed to be a transcript of Meirick MS. pedigree, commonly called the Cottrell Book, Vol. 2'.