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Student notes on petrology, 1903; university lectures and notes for lectures given at Aberystwyth and Manchester, 1919-[1930], and at Cambridge, 1931-1938; other lectures and addresses on geological subjects, 1925-1939; material relating to academic and consultative research, undertaken mainy in Wales, 1884-[1942], including material relating to the mineral mining industries and river drainage in Mid Wales; files of personal papers and correspondence, 1913-1943; copies of letters to his wife, 1909-1966; pocket notebooks, [1920s]-[1930s]; theses and papers by other individuals, 1931-1943; photographs and slides, [c. 1903]-[1949]; portfolios containing plans, sections, maps and graphs relating to mines, collieries and power stations in Wales and England, [c. 1871]-1935; miscellaneous papers and research notes, 1904-1966.

Manuscripts and papers of the families of Charles and Edwards, dated between [c. 1600] and 1922; they include letters from Thomas Charles Edwards to his wife, and their son Lewis Charles, 1876-1896; letters to Thomas Charles Edwards, 1885-1899; copies of letters, 1859-1898, including correspondence relating to University College of Wales, Aberystwyth; letters to and from Mary Roberts, 1867-[1893]; letters to their daughter, Elizabeth Alicia Edwards, 1887-1900; Edwards family letters, 1895-1900; and newspapers and press cuttings, [c. 1820]-1922.

A volume of notes taken by Timothy Lewis at Dr J. Gwenogvryn Evans's lectures on palaeography at the University of Manchester, 1906-1907 (ff. 20-56); Lewis's printed registration book for the University of Berlin, 1908 (ff. 57-68); and a manuscript 'Bibliography of Material relating to the History of Wales' in the hand of E[dward] A[rthur] Lewis, University College of Wales, Aberystwyth, 1900-1901 (ff. 1-19).
The registration book lists lectures to be taken, October 1908-March 1909 (ff. 59 verso-60), but is otherwise unused.

A holograph essay on 'Welsh Social Life as reflected in the Poems of Lewis Glyn Cothi' by 'Llynor' [E. Stanton Roberts]. The work was submitted for, and awarded, the T. E. Ellis Essay Prize at University College of Wales, Aberystwyth, during the Session 1909-1910.

A holograph essay on 'Y Mabinogion fel Llenyddiaeth' by 'Y Macwy Mud' [E. Stanton Roberts]. The essay was submitted in January 1911 for the T. E. Ellis Essay Prize at University College of Wales, Aberystwyth.