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Pocket notebooks kept between c. 1874 and c. 1901, many undated, containing adjudications by Gwilym Cowlyd on bardic competitions at various eisteddfodau, miscellaneous accounts, minutes of various committees, copies of poems and prose works, and a volume endorsed, 'Cymmrodoriaeth Barddas Glan Geirionydd. Gwilym Cowlyd's Book' and containing copious notes, poems and accounts for the years 1896 until 1901 on 'Arwest Geirionydd'.

Correspondence and papers relating mainly to Lord Hooson's political career, including papers regarding parliamentary questions, 1967-1978; the Welsh Liberal Party, 1963-1979; Montgomery County Liberal Association 1965-1979; Welsh Affairs, 1961-1978; University College of Wales, Aberystwyth, 1961-1968; Dyfed-Powys Constabulary, 1970-1976; foot and mouth disease in Wales, 1967-1968; transport problems in Mid-Wales, 1962-1974; National Theatre for Wales, 1968-1969; Rural Development Board for Wales, 1967-1970; Mid-Wales Hospital Service, 1972-1973; Farmers Union of Wales, 1966-1973; Aberfan Disaster, 1966-1967; television and radio reception in Wales, 1969-1976; Wales Tourist Board, 1968-1976; Plaid Cymru, Welsh nationalism, Welsh language, Devolution, Federalism, Welsh economy, unemployment, Rhondda West by-election, etc., 1960s-1970s; the Liberal Party correspondence, 1960s-1970s, Liberal Party organisation and policies, 1967-1971; Liberals and the Industrial Relations Bill, 1971-1973; Lib-Lab pact, 1977-1978; Liberal Foreign Affairs Panel, 1966-1967; NATO and the North Atlantic Assembly, 1966-1978; correspondence files of the Welsh Liberal Party, 1966-79; engagement diaries, 1966-1978; typescript speeches and notes for speeches, 1960s-1970s; parliamentary accounts, 1970-1972; miscellaneous speeches, press statements, newspaper cuttings, etc., 1960s-1970s; political papers [c. 1950]-1973, produced by various parties; Local Government Reform in Wales, 1993-1994; the Liberal Party's Pantyfedwen Conferences, 1956-1963; the London Welsh School, 1983-1993, the Llangollen International Eisteddfod, 1986-1997; the provision of speech therapy and physiotherapy in Clwyd, 1984-1990; constituency correspondence and papers, [1960]-1979; personal correspondence, 1965-1979; and correspondence, press releases and newspaper cuttings relating to Jeremy Thorpe, former leader of the Liberal Party, 1967-1979; together with papers relating to his business interests including, Laura Ashley Holdings Plc., 1984-1997; Severn River Crossing Plc, 1990-1997; and his legal career, 1949-1962. A further collection of Lord Hooson's papers were received in May 2011 - this group remains uncatalogued.

Papers of Thomas Owen ('Hesgin'), 1904-1956, comprising letters received, and copies of letters written by him to various newspapers and individuals, 1940-1956; literary compositions, including essays and short stories, submitted by him for competition at various eisteddfodau, including the National Eisteddfod of Wales; two volumes of autobiographical essays and reminiscences; nine volumes of press cuttings, mainly of articles by 'Hesgin' which appeared in newspapers and other publications, 1904-1956; scrapbooks and notebooks; and a minute book and other material relating to the Swansea district committee formed in connection with the National Petition for the Legal Recognition of the Welsh Language in Wales, 1938-1939.

Papurau Gwilym Wyn yn cynnwys barddoniaeth a rhyddiaith, beirniadaethau eisteddfodol, traethodau a nodiadau ar gyfer sgyrsiau a phregethau, [1852]-[1914] = Papers of Gwilym Wyn comprising poetry and prose works, eisteddfodic adjudications, essays and notes for talks and sermons, [1852]-[1914].

Drafftiau darlithoedd ac erthyglau gan G. J. Williams, ynghyd â nodiadau amrwyiol, yn ymwneud yn bennaf â'r Eisteddfod a'r Orsedd.

Llawysgrifau Evan James a James James, cerddoriaeth a barddoniaeth yn bennaf, 1806-1917, yn cynnwys fersiwn gwreiddiol yr alaw 'Glan Rhondda', y daethpwyd i'w hadnabod yn ddiweddarach fel Hen Wlad fy Nhadau, 1856; barddoniaeth Ieuan ab Iago,1831-1842; dyddiaduron,1806-1827, barddoniaeth, 1837-1849; cyfriflyfrau poced,1836-1837; a beirniadaethau eisteddfodol, 1853-1863. = Manuscripts of Evan James and James James, mainly music and poetry , 1831-1917, including the original version of the tune 'Glan Rhondda', which later became known as Hen Wlad fy Nhadau, 1856; poetry of Ieuan ab Iago, 1831-1842; diaries, 1806-1827, poetry, 1837-1849; pocket account books, 1836-1837; and Eisteddfod adjudications, 1853-1863.

Papurau, 1838-[1991], yn bennaf papurau personol a theuluol Eunice Bryn Williams, 1838-[1991], yn cynnwys darnau cerddoriaeth yn llaw Eunice Bryn Williams, 1954-[1980au]; nodiadau darlithoedd ar gerddoriaeth, [1940au-1980au]; papurau'n ymwneud â Chymdeithas Alawon Gwerin Cymru a Chymdeithas Cerdd Dant Cymru, [1950au-1980au], ac eisteddfodau, yn arbennig Eisteddfod yr Urdd, [1930au-1980au]; rhaglenni cyngherddau o gerddoriaeth Cymreig, 1939-1961; a gohebiaeth deuluol,1888-1961. = Papers, 1838-[1991], mainly personal and family papers of Eunice Bryn Williams, 1838-[1991], including music pieces in the handwriting of Eunice Bryn Williams, 1954-[1980s]; lecture notes on music, [1940s-1980s]; papers relating to Cymdeithas Alawon Gwerin Cymru and Cymdeithas Cerdd Dant Cymru, [1950s-1980s], and to eisteddfodau, especially Eisteddfod yr Urdd, [1930s-1980s]; concert programmes of Welsh music, 1939-1961; and family correspondence, 1888-1961.

Records and papers collected by Emrys Roberts, 1945-1983, including correspondence and papers relating to the National Eisteddfod, 1959-1976; the Development Board for Rural Wales, 1973-1981; and Wales (West and North) Television Ltd, 1960-1967. There are also papers relating to other committees on which Emrys Roberts sat, 1967-1983, and other miscellaneous papers, 1945-1981.

Press cuttings relating to Wales and Welsh culture, such as religion, politics, literature, music, education, St. David's Day celebrations and the Eisteddfod Genedlaethol, individuals, and the National Library of Wales [1895]-[1939].

Letters, 1902-1947, to D. R. Hughes; letters of literary interest, 1835-1902, collected by D. R. Hughes; material relating to the National Eisteddfod, 1881-1944, including poetry, 1881-1936; miscellaneous periodicals and books, 1904-1945; manuscript and newspaper cuttings belonging to the Rev. John Jones, Talysarn, Sir John H. Puleston and T. R. Roberts, [1857x1940].

A composite volume, lettered 'Eben Fardd's MS', comprising day and 'memoranda' books of Ebenezer Thomas ('Eben Fardd'). Among the material recorded by the writer are extracts relating to Tractarianism; diary entries, 1837-9, 1849; shop, school, bookbinding and other accounts, 1839-40; mensuration problems and tables, etc., c. 1834; 'Memorandum of Literary adventures and Transactions ... 1848-55, being largely a list of adjudications at eisteddfodau and literary meetings, and 'adjudicatory transactions conducted on the New Plan', 1855-6, and 'Requisitions & invitations declined', 1855-7; Llanarmon School, Clynnog School, and sundry accounts, 1827; etc.

A volume of miscellaneous press cuttings from Welsh and Welsh-American newspapers and periodical publications compiled, with some holograph annotations, by John Jones ('Myrddin Fardd'). The titles include 'Gorsedd y Beirdd', 'Yr Eisteddfod Genedlaethol' (Cardiff, 1883), 'Diwygiad yr Eisteddfod', 'Yr Eisteddfod a'i Hanes' (Rhyl, 1892), 'Llith Aneurin Fardd', 'Eisteddfod Genhedlaethol Aberdar, 1861 - "Hanes Llenyddol Cymru". Beirniadaeth' (by T. Stephens, Merthyr Tydfil), 'Sion Philip, Mochras', 'The British Kymry .... By the Rev. R. W. Morgan, Pc, Tregynon' (review), 'Yn y Bala', 'Review Flynyddol Gwirfoddolwyr Morgannwg ar Gomin Hirwain', 'Taith tua Chaerlleon-ar-Wysg', 'Y Gohebydd Gwibiol' (notes on the history and antiquities of Llandybie, Bettws, Llanarthney, Gelli Aur, Llanfihangel Aberbythych, Llangathen, Abergwili and Carmarthen), 'Hen Arferion Crefyddol y Cymry', 'Brawddegau y Werin' (a list of Welsh dialect expressions), etc. Also mounted in the volume is a printed prospectus of Robert Griffith (Manchester), Telyn a Cherdd Dannau y Cymry [?1913]. There are two labels laid on the outer upper cover, the one numbered '10' and the other in the hand of 'Myrddin Fardd' inscribed 'Chwidredd J. Morris Jones, Llythyrau Aneurin Fardd, Beirniadaeth T. Stephens, The British Kymry, etc. etc.'.

Papurau'r cymdeithasegydd Alwyn D. Rees, 1911-1974, yn cynnwys papurau'n ymwneud â Phrifysgol Cymru, yn bennaf â Choleg Prifysgol Cymru, Aberystwyth, 1920au-1974, gan gynnwys papurau'n ymwneud â'r comisiwn a sefydlwyd i archwilio strwythur ffederal Prifysgol Cymru yn y 1960au; papurau ynglŷn â lle'r Gymraeg yn y Brifysgol a'r ymgyrch i sefydlu neuadd Gymraeg i fyfyrwyr yn Aberystwyth,1967-1974; papurau'n ymwneud â llyfrau, erthyglau a darlithoedd Alwyn D. Rees, 1933-1973, a Chymdeithas yr Iaith Gymraeg, [c.1964]-1974; papurau'n ymwneud â Barn, 1966-1967; papurau'n ymwneud â darlledu yng Nghymru, 1938-1974; papurau'n ymwneud â'r diwydiant llechi yng Nghymru,1946; papurau'n ymwneud â gwleidyddiaeth yng Nghymru, 1911-1974; gohebiaeth gyffredinol, 1935-1974; a phapurau a gohebiaeth bersonol , 1930-1974 = Papers of the sociologist Alwyn D. Rees, 1911-1974, including papers relating to the University of Wales, mainly the University College of Wales, Aberystwyth, 1930s-1974, including papers relating to the commission established to examine the federal structure of the University of Wales in the 1960s; papers concerning the place of the Welsh language in the University and the campaign to establish a Welsh student hostel at Aberystwyth, 1967-1974; papers relating to the University of Malta, 1940-1951; Alwyn D. Rees's research papers, 1933-1973; papers relating to Alwyn D. Rees's books, articles and lectures, and further related research papers assembled by him, 1925-1974; papers relating to the Welsh language, 1952-1974, and 'Cymdeithas yr Iaith Gymraeg', [c. 1964]-1974; papers relating to 'Barn', 1966-1975; papers relating to broadcasting in Wales, 1938-1974; papers relating to the Welsh slate industry, 1946; papers relating to politics in Wales, 1911-1974; general correspondence, 1935-1974; and personal papers and correspondence, 1930-1974.