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Papers of Mary Garbett Edwards, including scrapbooks containing family photographs and letters, [1890]-1973; Montgomeryshire Liberal Party, General Purposes Committee, minute book, 1950-1959; letters, 1929-1983; journals of visits to North America, 1936-1949; notebooks and notes for speeches, [20th century]; radio scripts and related material, 1943-1963; papers relating to Garbett Edwards, including eisteddfod essays and other papers, 1897-[1930s], journal of Canadian visits, 1936-1939, and publications and annual reports of the Mid Wales Industrial Development Association, 1957-1973.

Papers, 1839-1931, relating to the Naylor family and the Leighton Hall and Brynllywarch estates, comprising accounts, rent schedules, valuations and sale catalogues, together with correspondence and other material relating to the family, and in particular to their activities as high sheriffs for Montgomeryshire.

Additional papers were received in July 2021, this material mainly comprising correspondence and newspaper cuttings, which trace the history of and events within the Naylor family and the Leighton Hall estate from the mid-nineteenth century to the near present day. The material includes a memorandum book, 1848-1856, belonging to John Naylor (1813-1889) of Leighton Hall.

Manuscripts, 1707-[1937], from the library of Richard Bennett of Llanbrynmair and Caersws, Montgomeryshire, much of which is in the hand of Richard Bennett himself. The collection comprises material largely of Montgomeryshire interest and includes parochial records, transcripts from parish registers, extracts from probate records (some of Merionethshire interest) and genealogical records, and extracts from printed works relating to Montgomeryshire.