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Papers, 1839-1931, relating to the Naylor family and the Leighton Hall and Brynllywarch estates, comprising accounts, rent schedules, valuations and sale catalogues, together with correspondence and other material relating to the family, and in particular to their activities as high sheriffs for Montgomeryshire.

Additional papers were received in July 2021, this material mainly comprising correspondence and newspaper cuttings, which trace the history of and events within the Naylor family and the Leighton Hall estate from the mid-nineteenth century to the near present day. The material includes a memorandum book, 1848-1856, belonging to John Naylor (1813-1889) of Leighton Hall.

Papers of John Sheringham mainly reflecting his research interests, including his research into Montgomeryshire place-names, 1980-1995, medieval Welsh history and laws, 1984-1995, and Breton history, 1988-1989; typescript notes on Welsh law, 1986-1990; typescript drafts of published works, and papers of the Machynlleth and District Civic Society, 1979-1993, and the Aberystwyth and District Civic Society, 1990-1994.

Papers, 1679-1983, of and accumulated by H. Noel Jerman, comprising: research papers, 1914-1975; files relating to his work in the Secret Intelligence services, 1941-1945; correspondence, notes and other papers relating mainly to archaeology, and also to his professional activities, 1948-1983; 'Notes and Memoranda' relating to events organised by the Cambrian Archaeological Association, 1883-1894; original records collected by him, 1679-1926, including deeds and documents relating to properties in Kerry, Montgomeryshire, 1679-1885, and Kerry School, 1843-1873, and copies of local newspapers, 1834-1868; records relating to the Dolforgan estate, including deeds and documents relating to properties in Montgomeryshire, Carmarthenshire and Merionethshire, 1807-1910, financial records, 1889-1939, and letter books, 1892-1930.

An additional consignment of materials of, and accumulated by, the late H. Noel Jerman (1909-1994), including his research papers relating to properties in Kerry and surrounding areas, papers relating to the Dolforgan estate, together with maps, sale catalogues, plans and photographs, and a lithograph of Dolforgan Hall by T. Way. This group remains uncatalogued.

Political correspondence and papers accumulated by Godfrey Lee, 1968-1988, relating to Plaid Cymru activities in Newport, 1968-1978, Plaid Cymru's Montgomeryshire branch, 1977-1988, and Welshpool branch, 1978-1980; the work of Gwent Regional Council [of Plaid Cymru], 1969-1977; together with Plaid Cymru Conference Programmes, 1969-1988; and literature concerning the Merthyr Tydfil by-election, 1972.

Deeds, 1555-1918, of clients and relating to properties in Cardiganshire, Merionethshire, Montgomeryshire and Radnorshire, including papers of the Penglais estate in the Aberystwyth area, 1555-1918; Aberystwyth borough records, 1759-1813; letters, 1794-1882; papers of John Parry, solicitors, Aberystwyth, including share certificates of the Aberystwyth Gas and Coke Company, 1839; Bwlch Consolidated Lead Mines, 1847; records concerning the Aberystwyth and Tregaron Bank, 1813-1844; miscellaneous papers, [c. 1783]-1932; printed items, [c. 1783]-1867; certificates of shares in the Aberystwyth Public Rooms, 1818-1821, and the Robinson Gold Mining Company, 1903; letters and papers relating to the estate of Roderick Richards, Penglais, [c. 1830]; builders' accounts, 1845; and tithe receipts, 1927-1932.

Title deeds and other documents, 1608-1794, relating mainly to properties in Montgomeryshire and Shropshire.

Deeds and documents, 1870-1907, concerning the estates of the Crewe-Read family of Llandinam Hall, Montgomeryshire.

Clement Davies's papers, [c.1884]-1967, mainly Liberal Party papers, 1928-1962, Clement Davies's political career, 1929-1965, Welsh affairs, 1936-1962, peace movements, 1940-1962, foreign affairs, 1944-1962, constituency papers, 1951-1962, and home affairs, 1953-1963; and papers and correspondence of Jano Clement-Davies, 1873-1969, and papers of Stanley Clement-Davies, 1920-1963.