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Large volumes, notebooks and folders, containing mainly poetry and prose compositions accumulated by various members of the Owen and Ormsby-Gore families, 1624-1868, and in particular by Frances Morres Gore, 1809-1832. The great majority are in English, but they include some works in French, Welsh, Latin and Italian by published and unpublished authors, including members of the Gore family. They broadly cover contemporary national events and politics of the Stuart period, the Hanoverian monarchy and the Napoleonic Wars, together with matters of local interest, and various romantic and moralistic themes.

Title deeds of properties belonging to the Llanddyn estate, situated mainly in Llangollen, Denbighshire, and in the adjacent parish of Rhiwabon, dated between 1498 and 1829.

Title deeds and other documents concerning properties purchased or leased by the Brogyntyn estate in the county of Merioneth, 1706-1961. They include a lease and arbitration award for Ty Cerrig, Talsarnau, in the parish of Llanfihangel-y-traethau, 1920-1961; miscellaneous properties in Llandanwg, Llanfihangel-y-traethau, Barmouth, Beddgelert, Harlech and other locations in Merioneth, 1706-1912; and mining and quarrying leases, 1837-1947.

Private letters, 1582-1933, written to, by or about individuals connected to the families of Maurice, Owen, Ormsby-Gore and Godolphin through marriage, friendship or business and a small number of items where neither the author nor the recipient can be identified. The group also contains several letters (mainly copies) by eminent figures of the Stuart period concerning matters of political and religious significance, which must reflect the interests of the Owen family and their associates.

Rentals and legal papers of miscellaneous manors, namely Aber and Cemais in Caernarfonshire and Anglesey, Whittington and Aston in Shropshire, 1591, 1632-1709, 1749-1774.

Miscellaneous papers, 1590-1938, deriving from the administration of estates in Caernarfonshire, Monmouthshire, Shropshire, Berkshire, Hertfordshire, Cornwall and elsewhere, where the provenance is unknown.

Title deeds and other documents relating to property owned by the Brogyntyn estate in Montgomeryshire, 1647-1902. One series concerns properties of the Penrhos and Cemmes (Cemais) estates, formerly belonging to John Owen, which descended to Mary Jane Ormsby Gore, 1647-1899; another series comprises records of the manors of Broniarth and Deuddwr, 1773-1894. Other deeds concern properties in the township of Broniarth in the parish of Guilsfield, 1740-1885, and at Sarnau in the parish of Meifod, 1828-1902.

Records deriving from administration of the Nant estate, lying mainly in Prestatyn in the parish of Meliden, Flintshire. They include a rental, [1380s], estate accounts, 1550-1675, and other estate administration papers, 1625-1685.

Title deeds of properties acquired through purchase, lease, mortgage, marriage and inheritance by members of the Conway and Mostyn families of Nant, [mid-14 cent.], 1367-[c. 1686], mainly in the parishes of Cwm, Llanasa, Meliden and Rhiwlyfnwyd, but also in Bodfari, Gwaunysgor, Cilcain, Rhuddlan and Whitford. The earliest title deeds include a small number of fourteenth century documents involving the de Crevecoeur family, lords of Prestatyn. Further items of significance are conveyances of lands in Cwm and Diserth from 1533 to 1625 by the Lloyds of Hiraddug, who had established a marital connection to the Mostyn family. Other deeds show the acquisition of land by the Conway family, mainly in Llanasa and Meliden, between 1539 and 1624. Family settlements and associated documents of the Mostyn family, dating from 1625 to 1659, relate to lands mainly in Meliden, but also in Llanasa, Cilcain, Cwm and Whitford. Other families represented in the deeds include Holland of Prestatyn, and Prestland of Prestatyn and Wardle, Cheshire.

Complete editions, cuttings and pages of newspapers, 1685-1887; printed newsletters, broadsides, advertisements and general information leaflets, 1666-1861; and manuscript newsletters, 1676-1710.

Manuscript and printed papers of academic and general interest collected or researched by the family, comprising original documents [14 cent.], 1590, sermons [early 17 cent. x mid 18 cent.], epitaphs, [c. 1686], 1736, prophecies, [c. 1694], [19 cent.], catalogues of books and documents, including Brogyntyn library, 1702-1946, various academic exercises, notes, articles and other literature relating to religion, historical and antiquarian subjects, literature, natural history and topography, philosophical and moralistic themes, money and other subjects of general interest, [1656]-1940.

Personal papers, being journals and diaries of Emily Charlotte Seymour (married name Ormsby-Gore, second Lady Harlech), 1844-1849, 1890, some of which describe travels with her family to Chile and elsewhere in South America, and including a diary of her mother, Georgiana Mary Seymour, 1869-1870.

Personal papers, comprising diaries and army papers of George Ralph Charles Ormsby-Gore, third Baron Harlech, 1873-1883, and diaries of his wife Margaret Ethel, 1914-1937.

Personal papers of William George Arthur Ormsby-Gore, fourth Baron Harlech, comprising notes on church architecture and art, 1903-1927; addresses and essays deriving from both his professional career and his personal interest in (mainly) European art, 1925-1945; and miscellaneous papers relating to his education, personal life and work abroad, 1904-1943.

Personal papers associated with the career and interests of William Ormsby-Gore, 1822-1860.

Personal papers of William Richard Ormsby-Gore, second Baron Harlech, consisting of diaries, 1837-1893, and papers relating to his career and interests, 1836-1894. They cover aspects of his travels in Europe, his army career and participation in the Crimean War, official business as an Irish MP, involvement in local institutions and his membership of the freemasons in North Wales and Ireland.

Personal papers of the Owen and Godolphin families and various members of the Ormsby-Gore family, comprising almanacks and pocket books, 1676-1765, and miscellaneous papers relating to personal interests, physical statistics, training, education and careers, 1672-(Watermark 1860), 1893-[1900].

Original and copy wills, administration bonds, occasional inventories and other documents associated with probate belonging to the main families of Maurice of Clenennau, Owen of Clenennau and Brogyntyn (Porkington) and Ormsby-Gore of Brogyntyn, 1621-1829, and those who were connected with them by marriage, namely Anwyl of Park, 1600-1700, Godolphin of Abertanat, 1725-[c. 1862], Vaughan of Corsygedol, 1606, 1636, and Wynn of Glyn, Sylfaen and Ystumcegid, 1563-1682.

Rentals of various parts of the Brogyntyn estate in Merioneth, Caernarfonshire, Shropshire, Denbighshire and Montgomeryshire, 1795-1913; and memoranda and reports on the rentals and accounts, 1834-1926.

Title deeds and other documents relating to properties mainly in the parishes of Oswestry, Selatyn and Whittington in the county of Salop (Shropshire), either purchased by the Brogyntyn estate or already owned and later sold or leased by them, 1607-1939. The properties include lands which formerly belonged to the Earls of Powis, the Lloyd family of Aston and the Owen family of Woodhouse, former common lands in the manor of Whittington and the Drenewydd estate purchased from the Wynne family of Peniarth in 1830. There are substantial quantities of deeds for the farm of Pentreclawdd, 1607-1899, the Vron, Selatyn, 1697-1874, Pentre David, 1707-1827, Pentrepant, 1741-1894, lands around the Brick Kilns in Oswestry, 1783-1909, and miscellaneous other properties, 1740-1939.