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Letters, 1778-1814, from Thomas Charles to Sarah Jones, who became his wife in 1783, from Sarah to Thomas Charles, and from Thomas Charles to his son Thomas Rice and daughter Maria; letters addressed to Thomas Charles by various friends and collaborators; a receipt from John Roberts to Sarah Jones, 1773; a letter from Richard Lloyd, Beaumaris to Thomas Rice Charles, 1815; other papers.

Miscellaneous papers of the Charles family, including an example of the autograph of Maria, wife of Thomas Rice Charles (son of Thomas Charles of Bala); a copy of a licence to John Davies, Fronheulog to print 2,300 copies of Thomas Charles's dictionary, 1818; letters to David Charles, Trefeca from David Charles, Carmarthen, 1833-1834, and from Lewis Edwards, Edinburgh, 1836; a copy of the marriage certificate of Thomas Charles and Celia Browning, 1835; a letter from David Charles to Robert Saunderson, Bala concerning Thomas Charles's dictionary, 1840; papers relating to the 'Charles Trust', 1858-1859; papers relating to the purchase of Leaden Hall, Aberdyfi by David Charles, 1874; papers relating to the ship Maglona of Aberdyfi, 1876; autobiographical notes and miscellanea by David Charles, 1833-1878, and press cuttings, including biographical material relating to him.