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Personal correspondence, 1916-1954; study notes, 1902-1952; biographical material, 1903-1954; notebooks entitled 'Tennyson Biography'; sermons and addresses, 1932-1952; orders of service for Victory, 1945, the United Nations 1946, Human Rights Day, 1951-1954, the Coronation and other occasions, 1931-1954; religious and international affairs, 1944-1945; Welsh Book Festivals, 1935-1938; Welsh School of Social Service, 1911-1940; The Gregynog Conferences on International Education, 1922-1937; Advisory Education Committee minutes, 1926-1929; international co-operation, 1933-1937; Welsh nationalism, 1910-1943, including nationalists' attitudes towards World War II, 1939-1941; broadcasting materials mostly of Marconi and Kemp, 1931-1953; Welsh broadcasting, 1923-1948; the Welsh Children's Peace Message, Pageant, and Wales and the Peace Movement, 1923-1955; BBC staff changes and administration in Wales, 1934-1952; the League of Nations, 1923-1952; the Welsh National Council of the League of Nations Union, 1923-1945; United Nations, 1942-1954; UNESCO, 1925-1947; addresses, radio talks and notebooks on the international situation, 1930-1954; Council for Education in World Citizenship, 1940-1950; London International Assembly, 1941-1944; Welsh Committee of the UNESCO, 1949-1953 and human rights materials, 1945-1953.

Papers of Sir Rhys Hopkin Morris, 1921-1940, comprising his diary, 1928, whilst a member of the Parliamentary Delegation to Tanganyika; material relating to the Parliamentary Commission on the Palestine Disturbances, 1921-1930; and duplicate typescript Daily Digests of foreign broadcasts prepared by the Monitoring Service of the BBC, 1939-1940. No material concerning the Liberal Party is included.

Papers of Wynford Vaughan Thomas, 1850-1986, including war despatches, 1943-1945; papers relating to Indian independence, 1947; scripts of radio programmes on the Middle East, 1956; papers relating to state occasions, 1950-1956; notes for a proposed book on the river Niger, 1961-1963; manuscript and typescript copies of stories, articles, lectures, etc., 1947-1964; scripts of radio and TV programmes and proposed programmes, 1946-[1980s]; notes for proposed works on autobiography, 'Journeys', the River Niger, and Welsh history, [1950s]-1984; manuscripts, notes and typescripts for the published works Anzio, Madly in all directions, Shell Guide to Wales, Portrait of Gower, and Trust to talk, 1958-1980; travel journals, 1947-1964, recording visits to India, West Indies, Europe, Middle East, Africa and Hong Kong and Singapore; notebooks containing notes, drawings and miscellanea, [1947]-[1960s]; financial papers, 1945-1973; correspondence, 1936-1986; papers relating to wine, 1980-1984; papers relating to Dylan Thomas and his literary estate, 1955-1974; family papers, 1895-1950; press cuttings relating to his broadcasting career, 1937-1978; papers relating to Botticelli's painting, 'Primavera', 1945-1988; and miscellaneous papers, mainly printed, 1850-1974.