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The collection comprises volumes of primary records, 1922-1950, (including executive committee minutes, north Wales committee minutes, finance committee minutes, cash books, ledgers, campaign committee minutes, general purposes committee minutes); the records of the Welsh National Council of the League of Nations Union, 1920-1945; minutes of the committees of the League of Nations Union, 1925-1939; minutes of the sub-committees of the League of Nations Union, 1927-1942. Secondary records of the League of Nations Union: general meetings, 1928-1938; national meetings, 1928-1937; conferences, 1922-1937; committees, 1922-1938; financial records, 1925-1938; educational records, 1922-1946; publications, 1923-1932; publicity, 1929-1947; personal files, 1922-1939; enquiries, 1922-1938; formation of branches, 1923-1938; reports, 1924-1938; London headquarters, 1923-1938; general files, 1922-1951. Branch files, 1922-1940; weekly returns relating to membership etc., 1922-1934; membership, county files etc., 1930-1938; Headway notes, correspondence, press cuttings etc., 1922-1938; League of Nations Union miscellaneous papers, 1923-1939. United Nations Association general files, 1943-1954; United Nations Association committees, 1943-1965; United Nations Association sub-committees, 1947-1952; UNA finance, 1940-1961; UNA membership, 1946-1964; UNA accounts, 1951-1960; UNA 'Files from a series designated letter/number', 1961-1967; UNA branches, 1943-1950; League of Nations Union/UNA meetings, 1944-1964; Temple, 1939-1957; personal files, 1943-1950s; educational themes, 1944-1950; Newsletters, 1961; UNA conferences, 1962-1967; UNA campaigns, 1964-1966; Youth against Humger/Council for Education in World Citizenship Competitions, 1965-1967. Goodwill message: replies to children's wireless message (CWM), 1925-1929; replies to CWM, 1930-1938; CWM related material, 1935-1938; material relating to World Children's Message up to 1939, arranged by countries, 1927-1938; replies to CWM, 1939, arranged by countries; CWM lists of replies, 1928-1939; WCM, copies of replies, correspondence etc., 1938-1959.

Personal correspondence, 1916-1954; study notes, 1902-1952; biographical material, 1903-1954; notebooks entitled 'Tennyson Biography'; sermons and addresses, 1932-1952; orders of service for Victory, 1945, the United Nations 1946, Human Rights Day, 1951-1954, the Coronation and other occasions, 1931-1954; religious and international affairs, 1944-1945; Welsh Book Festivals, 1935-1938; Welsh School of Social Service, 1911-1940; The Gregynog Conferences on International Education, 1922-1937; Advisory Education Committee minutes, 1926-1929; international co-operation, 1933-1937; Welsh nationalism, 1910-1943, including nationalists' attitudes towards World War II, 1939-1941; broadcasting materials mostly of Marconi and Kemp, 1931-1953; Welsh broadcasting, 1923-1948; the Welsh Children's Peace Message, Pageant, and Wales and the Peace Movement, 1923-1955; BBC staff changes and administration in Wales, 1934-1952; the League of Nations, 1923-1952; the Welsh National Council of the League of Nations Union, 1923-1945; United Nations, 1942-1954; UNESCO, 1925-1947; addresses, radio talks and notebooks on the international situation, 1930-1954; Council for Education in World Citizenship, 1940-1950; London International Assembly, 1941-1944; Welsh Committee of the UNESCO, 1949-1953 and human rights materials, 1945-1953.