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Papers of Stuart Rendel and family members, including papers relating to the University College of Wales, Aberystwyth, and the proposal to establish the National Library of Wales and its development during the early years of its existence, 1883-1916; speeches, addresses and political papers relating to disestablishment of the church in Wales and the 1889 Intermediate Education Act, 1882-1909; press cuttings, 1881-1913; photographs, 1892; miscellaneous letters, 1878-1912; letters to Stuart Rendel, 1853-1912, including letters from A. C. Humphreys Owen, 1877-1905, family letters, 1853-1902, and letters from prominent political figures and Welsh public figures; letters and copies of letters from Rendel, 1880-1912; diaries, mainly recording details of Stuart Rendel's business activities, 1863-1869; notes of conversations with W. E. Gladstone, John Morley and H. H. Asquith, 1888-1910; papers relating to Chinese affairs and French and Chinese peace talks, 1884-1886; papers of James Meadows Rendel, including letters, 1828-1856, and papers relating to his estate, 1856-1859; letters of Catherine Jane Rendel, 1845-1855; letters and papers of George Wightwick Rendel, 1871-1902; papers relating to Rendel's other brothers, 1841-1889, and his daughters, 1882-1910; letters and papers of Harry Stuart Goodhart-Rendel, 1898-1959, and other papers concerning him, 1963-1977; papers, mainly letters, of the Goodhart family, 1819-1957; papers of Miss Rosemary Rendel, 1986-1996; papers of Sir George William Rendel, including: Foreign Office papers, 1917-1967, correspondence, 1912-1973, papers relating to the Catholic Union of Great Britain, 1942-1979, lectures, diaries and notes, 1915-1954, personal and family papers, 1908-1980, and material relating to the book The Sword and the Olive (1957), 1954-1986.

The second of three volumes containing some one hundred and eighty-eight letters, 1856-1888, addressed to Henry Richard and dealing particularly with politics, the peace movement, education and other affairs in Wales.
The correspondents include Henry Fawcett, (Mrs) M. G. Fawcett, Dudley Field, Hugh Fielden, Lord [Edmond] Fitzmaurice, W. E. Forster, W. H. Fremantle, Joseph F. B. Frith, Thomas Gee, H. M. Milner Gibson, J. H. Gladstone, W. E. Gladstone, Granville George [Leveson-Gower], second earl Granville, John Griffith (Y Gohebydd), Lord Richard Grosvenor, first baron Stalbridge, George Hadfield, John Hampden (Croydon), Sir William Harcourt, H. D. Harper (Jesus College, Oxford), Thomas Harris, Arthur Hobhouse, Alfred Illingworth, Basil M. Jones, J. Viriamu Jones and Michael D. Jones.

An extract from the minutes of the Council of the University College of Wales, 30 June 1870, relating to an interview between Henry Richard and W. E. Gladstone on the subject of an Exchequer grant to the College (item 1); and a draft (or copy) of a letter, 4 July 1883, from Henry Richard (item 2) and of a statement on intermediate education in Wales, signed by nearly all the members of Parliament for Welsh constituencies, to be sent to Mr Gladstone (item 3).