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Manuscript collections containing original and transcribed poetry and prose, 1543-[20th century]; religious works, 1611-1914; biographies, chronicles, archaeological and historical notes, works on travel, folklore, recipes, grammars, vocabularies and philological notes, 1673-1900; rent-rolls, parish registers, tithe account books, bidding books, minute books and registers of various societies, 1608-1863; pedigrees and genealogical notes, [17th century]-1871, commonplace books, [18th century]-1904, volumes of press-cuttings; manuscripts in the hand of J. H. Davies, including transcripts of and indexes to Welsh poetry, bibliographical notes, literary and legal extracts, pedigrees, biographical data and notes on place-names, 1891-1923; autograph letters from prominent Welsh literary figures, 1674-1921; autograph manuscripts of John Jones, Gellilyfdy, Dafydd Ellis of Criccieth, Eben Fardd (including diaries, 1836-1859), Peter Williams, D. Silvan Evans, Thomas Richards and Myrddin Fardd.

Genealogical material compiled for Lord Howard de Walden during the early years of his tenancy of Chirk Castle, comprising transcripts of manuscripts containing Welsh genealogies compiled under the supervision of Arthur Owen Vaughan ('Owen Rhoscomyl'); letters, 1906-1921, mainly addressed to Arthur Owen Vaughan, relating to antiquarian and genealogical matters, academic research, etc.; genealogical notes, pedigrees, transcripts of wills, etc.; and an account book, 1870-1872, of the Chirk Castle Estate.

Manuscripts, [late 12 cent.]-[early 20 cent.], formerly part of the library of the Mostyn family of Mostyn Hall, Flintshire, comprising transcripts and extracts from Giraldus Cambrensis, Geoffrey of Monmouth, Dares Phrygius, Nennius, Gildas, David Jenkins (Judge Jenkins), Sir John Wynn of Gwydir, Lydgate's 'Life of Our Lady', Leland's Itinerary, 'Chroniques de France', historical manuscripts such as Brut y Tywysiogion and Brut y Brenhinoedd, Welsh romances and the Mabinogion; collections of mainly Welsh poetry, among them the seventeenth-century volumes Llyfr Coch Nannau and Llyfr Gwyn Corsygedol, containing poems by Dafydd ap Gwilym, Guto'r Glyn, Tudur Aled, Siôn Cent and others; genealogies, pedigrees and histories; official papers relating to Caernarvonshire; catalogues of the Mostyn and Gloddaeth libraries, 1692-1842; etc.