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Music manuscripts and papers, [c. 1750]-1945, including hundreds of folk songs brought together by Dr J. Lloyd Williams in his role as Editor of the Welsh Folk-Song Society, and papers relating to his researches into the history of Welsh music; material relating to his interest and vocation in the field of botany, 1871-1942; and personal papers, [?1870]-1946.

A collection of hymn-tunes and other pieces composed in the second half of the nineteenth century by William Evans Alaw Afan.