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Records relating mainly to the industrial concerns of the Crawshay family of Cyfarthfa, Merthyr Tydfil, Glamorgan, [1706]-1878, including leters and letter books of William Crawshay I and II and Robert Crawshay, 1806-1877; cash books, ledgers and bankers drafts, 1834-1888; deeds, [1706]-1885; wills, deeds and miscellaneous material, 1801-1838; balance sheets for ironworks, 1810-1867; will, valuation and probate for William Crawshay II, 1865-1869; shares and bills of exchange, 1870-1878; and Hilston Park estate papers, 1838-1862 and Caversham Park estate papers, 1826-1864. The archive represents the working papers of a major ironworking dynasty.

Papers of, and acquired by, the Welsh Church Commission, 1283-1960, including records of the Commission, 1914-1960; records relating to border parishes, 1914-1915; accounts, 1920-1958; papers relating to Sir Alfred Watson, 1916-1941; records concerning compensation to lay holders of freehold offices, 1915-1931; records relating to burial grounds, 1934-1947; records relating to the destination of records, 1914-1960; records relating to parish lands, 1844-1946; manorial records and court books, 1842-1925; transfer of documents, 1822-1947; deeds of properties, 1566-1929; and rentals and surveys, 1919-1947.

Cofnodion Plaid Cymru, 1915-1999, yn cynnwys cofnodion, agenda and gohebiaeth y pwyllgor gwaith a phwyllgorau eraill, 1925-1997; gohebiaeth gyffredinol, 1925-1998, gyda nifer o aelodau a swyddogion blaenllaw y blaid; cofnodion, gohebiaeth a phapurau eraill y gwahanol bwyllgorau rhanbarthol, 1925-1997, a changhennau,1930-1992; cofnodion a dogfennaeth y Cyngor Cenedlaethol, 1967-1997; cofnodion ariannol, yn cynnwys rhai papur newydd misol y blaid Y Ddraig Goch a Welsh Nation a Chronfa Gŵyl Ddewi, 1927-1996; rhaglenni a threfniadau ar gyfer cynadleddau ac Ysgolion Haf, 1933-1998; cofnodion aelodaeth, 1930-1996; papurau y Grŵp Ymchwil, [c.1960]-1995; papurau, yn cynnwys areithiau ac effemera, yn ymwneud ag etholiadau, 1929-1999; papurau yn ymwneud ag Adran y Menywod, 1924-1996, a'r Mudiad Ieuenctid, 1964-1998; papurau yn ymwneud â refferendwm datganoli 1979,1969-1983, a refferendwm 1997, a Chynulliad Cymru,1992-1998; papurau yn ymwneud â Y Ddraig Goch, Welsh Nation a chyhoeddiadau eraill, 1932-1996; deunydd printiedig gan Blaid Cymru ac eraill yn cynnwys llyfrau, cyfnodolion a phamffledi,1913-1996; torion o'r wasg, 1924-1996; cylchlythyron, 1938-1992; papurau yn ymwneud â'r Blaid Seneddol,1980-1996; papurau unigolion ac rhai ar wahanol bynciau amrywiol, 1926-1998 = Records of Plaid Cymru, 1915-1999, including minutes, agendas and correspondence of the executive and other committees, 1925-1997; general correspondence, 1925-1998, with many prominent party members and officials; minutes, correspondence and other papers of the various regional committees, 1925-1997, and branches, 1930-1992; minutes and records of the National Council, 1967-1997; financial records, including those of the party's monthly newspaper Y Ddraig Goch and Welsh Nation and Cronfa Gwyl Dewi, 1927-1996; arrangements for and programmes of conferences and Summer Schools, 1933-1998; membership records, 1930-1996; papers of the Grŵp Ymchwil (research group), [c.1960]-1995; papers, including speeches and ephemera, relating to elections, 1929-1999; papers relating to the Adran Menywod (Women's Section), 1934-1996, and the Mudiad Ieuenctid (Youth Movement), 1964-1998; papers relating to the 1979 devolution referendum, 1969-1983, and the 1997 referendum and Welsh Assembly, 1992-1998; papers relating to Y Ddraig Goch, Welsh Nation and other publications, 1932-1996; printed matter by Plaid Cymru and others including books, periodicals and pamphlets, 1913-1996; press cuttings, 1924-1996; circulars, 1938-1992; papers relating to the Parliamentary Party, 1980-1996; papers of individuals and to various miscellaneous topics, 1926-1998.