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Papers and other material relating to the personal life and professional career of the Welsh actress Siân Phillips, which include material relating to her early education and training and to her subsequent many and varied stage and screen rôles; correspondence from family members and from her myriad friends and colleagues in the world of theatre and film; press articles, etc relating to her stormy marriage to legendary actor Peter O'Toole; notebooks and diaries containing day-to-day schedules and personal reflections; and the copious preparatory material which went into the publication of her two-volume autobiography, Private Faces (1999) and Public Places (2001).

Material donated March 2023, which includes diaries, notebooks and press cuttings, have been amalgamated within the existing archive.