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Manuscripts and papers of the families of Charles and Edwards, dated between [c. 1600] and 1922; they include letters from Thomas Charles Edwards to his wife, and their son Lewis Charles, 1876-1896; letters to Thomas Charles Edwards, 1885-1899; copies of letters, 1859-1898, including correspondence relating to University College of Wales, Aberystwyth; letters to and from Mary Roberts, 1867-[1893]; letters to their daughter, Elizabeth Alicia Edwards, 1887-1900; Edwards family letters, 1895-1900; and newspapers and press cuttings, [c. 1820]-1922.

General correspondence files, chiefly financial in nature, with various companies, related bodies such as National Association of Agricultural Services, etc., 1955-1979, correspondence with Ministry of Agriculture and Fisheries, 1930-1957; Ministry of Agriculture, Fisheries and Food, 1957-1968; Agricultural Research Council, 1951-1979; National Institute for Agricultural Botany, 1954-1985; WPBS reports, 1919-1980; annual reports, 1944-196; papers of the Directors and heads of sections, 1919-1974; minutes, etc., relating to various seed production committees, 1947-1957; the papers of Gwilym Evans, 1928-1961; the Cahn Hill Improvement Station at Pwllpeiran, Cwmystwyth, 1933-1973; files of experiments, with details of experiments in progress, field record cards, slips and notebooks, agrotype experiment data, including results of research undertaken at Bicton, Cambridge, Newcastle, Hurley and Aberdeen, and at Welsh county trials, [1919]-1969.