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Records relating to the administration of the diocese of Llandaff and Dean and Chapter of Llandaff Cathedral from the seventeenth century, comprising episcopal registers, bishops' transcripts, marriage bonds and affidavits, and chapter act books, as well as records relating to: the ordination, appointment and resignation of clergymen and other individuals; the licensing of curates and other individuals; the licensing and consecration of land and buildings; faculty papers; dilapidations and sequestrations; augmentations, the creation of new parishes and boundary changes; dissenters' meeting houses; episcopal revenues and accounts; charities; parochial returns; deeds; consistory courts; visitations; correspondence; and miscellaneous volumes and papers.

Additional papers of the Diocese of Llandaf comprising the Bishop's Visitations for 2002 and 2006 - 9 large archive boxes in April 2015.

Additional records of the Diocese of Llandaff, 1923-2012, including Archdeacon’s Visitations, 2009-2012; Marriage Licences, 1988-2011; and Ordination papers, 1988-2001 - 10 large archive boxes in December 2015.

Additional papers comprising faculties, 2011-2016, together with two documents, 1921 and 1940, and a photograph relating to the Church of St Theodore, Bryncethin (February 2017); faculties and Archdeacons Returns (April 2017); and faculties (August 2017).

Further records comprising two boxes of Faculty papers, 2007-2018, and three boxes of Archdeacons returns (including parish reports and accounts), 2013-2015; February 2020.

Two further boxes containing Grants of Faculty, 2008-2019; November 2022.

A folder containing Faculty papers for Llangynwyd, Hirwaun and Porth; March 2023.

A small bundle of Faculty papers for Pwllgwaun and Llandaff Cathedral; May 2023.

Records of Margam Rural Deanery, 1969-1993, consisiting of minutes of Chapter meetings, correspondence of the Chapter Clerk, and other records relating to the organisation and financing of meetings; June 2026.