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Manuscripts once held in the library of Plas Llanstephan, Carmarthenshire. The collection comprises mainly transcripts from medieval Welsh manuscripts such as the Red Book of Hergest, the Black Book of Carmarthen and the Red Book of Talgarth which include poetry, triads, pedigrees, arms, lives of saints, Brut y Brenhinedd, Brut y Tywysogion, the Laws of Hywel Dda, etc.; grammars and vocabularies; translations, mainly from Latin and English sources; proverbs; theological tracts; medical recipes; etc. The earliest of the manuscripts date from the thirteenth to the fifteenth centuries. Most of the manuscripts are in the hands of Moses and Samuel Williams, with other scribes including Dr John Davies, Mallwyd, Dr John David Rhys, William Maurice, 'Iaco ab Dewi', Edward Lhuyd and William Owen-Pughe.

'Y Llyfr hir or Mwythig', being a collection of five hundred and sixty-six cywyddau, etc. by various authors arranged into 'books' according to subject. The poems in each 'book' are numbered separately. The poets cited include Iolo Goch, Dafydd ap Gwilym, Siôn Cent, Iorwerth Fynglwyd, Bedo Brwynllys and Siôn Phylip. The volume is dated temp. James II (see p. 382). The text is followed by nine folios of index, arranged under authors' names, by Richard Morris. Following the index are three further poems (by Dafydd ap Gwilym, Siôn Cent and Dafydd ab Edmwnt) in the hand of the Reverend Samuel Williams.
The volume is in the same hand as Llanstephan MSS 47, 48 and the end of 164.

A manuscript containing prophecies in prose and verse and including alleged prophecies of Myrddin and Taliesin and the works of Iolo Goch, Dafydd Llwyd and Rhys Nanmor.
The text at p. 39b is said to be 'copied out of the Chronicle of Guttun Owain'. The text at the end beginning 'Proffwydoliaeth Banastr o Brydain fawr ...' is continued on p. 13 of the manuscript.

A manuscript, probably in the hand of David Parry (certainly pp. 353-367 are in his writing, and cf. Llanstephan MSS 138, 147, 148) and written c. 1640 (see p. 360) containing Dares Phrygius; Geoffrey of Monmouth's Historia; Brut y Tywysogion; Cantreds and Commotes of Wales; Brut y Saeson; 'O oes Gwrtheyrn', etc.; Imago mundi; Buchedd Silvester; and poetry (cols 1396-1442, 1357-1361). This is followed by 'Meddyginiaeth', etc.; 'Music Telyn a Chrwth'; 'Englynion i Dduw ar byd by W. Cynwal'; the names of the Lord Chancellors of England, of the Bishops of Bangor down to William Roberts (bishop from 1637 to 1665), and of the Lord Presidents of Wales to John Egerton, Earl of Bridgewater (President from 1631 to 1642); followed (pp. 362-368) by poetry from a manuscript in the possession of Roger Salesbury of Rhug, the poets cited including Taliesin and Rhys Fardd.
Pp. 1-351 are copied from the Red Book of Hergest.

A manuscript containing transcripts by David Parry from the Red Book of Hergest, together with other poetry, the volume being compiled before it was given to Jesus College, Oxford in 1701. The contents of the volume are as follows: A Welsh Grammar copied from the Red Book of Hergest (col. 1117), with collations by Samuel Williams from Llanstephan MS 3, p. 472 (original foliation I-Vb, 1-7); a copy of the poetry on cols 1143-1356 of the Red Book of Hergest (original foliation 7-12b, original pagination 13-168, 169-265); followed by sixteen leaves at the end of the manuscript containing poems by Robin Ddu o Fôn, Tudur Aled, Rhys Nanmor and others, together with the pedigree of Sir Rhys ap Thomas.
Samuel Williams has copied a good many of the older material in a modernised orthography on the side left blank by the original copyist. There are also marginalia in the hand of Moses Williams. A note, probably in the hand of Samuel Williams, on p. 265 (original pagination) reads 'All the Poetry collated March 27 . 1722'.

Copies made from the Red Book of Hergest by David Parry in 1697 (see f. 202), written mostly on one side only. The volume contains De Carolo Magno (ff. 7-77); Historia Caroli Magni (ff. 78-91); Imago Mundi (ff. 91-98); Brief Chronicle (f. 98 = cols 516-518 of the Red Book of Hergest); Cato Cymraeg (ff. 100-104 = cols 520-527 of the Red Book of Hergest); Breuddwyt Ronabwy (ff. 104-113); Proffwydolyaeth Sibli Doeth (ff. 114-119); Kyvoessi Myrdin etc. (ff. 120-125 = cols 577-584 of the Red Book of Hergest); 'Proff: yr Eryr, Pan aeth llu i lychlyn, Enweu ynys prydein etc.' (ff. 125-129); Iarlles y Ffynnawn (ff. 130-147); Peredur (ff. 147-172); Amlyn ac Amic (ff. 172-187); poetry (ff. 188-199 = cols 1366-1396 of the Red Book of Hergest); and Y Mab Cric Iustus llwyt (ff. 200-202 = cols 1362-1367 of the Red Book of Hergest). This text is followed by sayings of 'Cattwn ddoeth', Taliesin, etc. (f. 203); 'Breuddwyd Gron: Ddu' (f. 203); triads (ff. 204-207); and poetry by Lewis Glyn Cothi, Lewys Morganwg and others (ff. 208-214).

A manuscript containing 'A Short History of Wales' 'copied from a MS. in the study of Mr. Edwards of Rhyd y Gors near Caermarthen'.

A manuscript containing poetry by Dafydd ap Gwilym, Guto'r Glyn, Dafydd ab Edmwnd and others (pp. 1-102 (the text beginning at p. 99 being a fragment only)); and Myrddin's 'Vaticinium' (pp. 131-146).
The manuscript is written in three different hands: pp. 1-102 belong to the third quarter of the sixteenth century; pp. 103-130 to the fourth quarter of the sixteenth century; and pp. 131-146 are in the hand of Sir Thomas Wiliems in his earliest style, c. 1576.

A manuscript containing poetry of Taliesin, Iolo Goch, Edmwnd Prys, Dafydd ab Edmwnd, William Phylip and others.
The manuscript is written in many hands but mostly in that of T. Jones of Pennant Melangell (see p. 222), c. 1680 (see pp. 76, 81).

A manuscript containing Brut y Tywysogion. Ff. 1-111, 114-121 are in the autograph of Richard ap John of Scorlegan, Llangynhafal.
The text is a copy of Mostyn MS 116 when that manuscript was complete.

A manuscript containing cywyddau brud and other poetry (pp. 7-8, 13-78, 87-94, 101-111, 115-130, 135-136, 154-298), the poets cited including Taliesin, Dafydd Nanmor, Dafydd ab Edmwnd and Siôn Tudur; prophecies of Merlin (pp. 79-86, 112-114, 131-134, 137-140); two imperfect documents of the Bishops of St Asaph and Gloucester, dated 1627 and 1596 (pp. 9, 11); 'Swynion a Meddeginiaetheu'; &c.

A manuscript written in two hands containing Historia Brittonum, et Cronice de Gestis ac Nominibus Regum Anglie. Beginning at p. 132 is a brief continuation of the Chronicles down to Henry VI in a later hand.

A manuscript containing the rentals and estate memoranda of Maurice Wynn of Gwydir; together with the stock accounts of several farms.
Among the losses of one farm's stock in the year 1570 is a sheep 'killed by an eagle' (p. 77).

A notebook of Edward Lhuyd, written 1698 (see pp. 10, 52), containing details of monumental inscriptions in Llanboidy (p. 6), Defynnog (p. 7), Llanfihangel (Mongomeryshire) (p. 17), Trawsfynydd (p. 31), Llangadog (p. 53), Herefordshire (pp. 58, 72), Llanllywenfel (p. 75), Llanafan Fawr (p. 77) and Llandanwg (p. 89); sketches of stone crosses (pp. 59-61, 73), stone circles (pp. 27, 44, 94, 99, 100) and further stones (pp. 2, 9, 42-3, 56), lime pit fossils (pp. 14, 44, 54, 62, 84-5, 145), a window (p. 3), Llangorse lake (p. 36), and the shore by Barry Island (pp. 37-8); and details of tombstones and their epitaphs (pp. 4, 11, 13, 39, 47, 63, 69, 81). The volume also includes notes relating to manuscripts and their owners (pp. 65-74), etc. An autograph note on p. 120 states: 'Mr. Edward Lhwyd was born at Lappiton parish, his nurse is now [?1698] living at Krew green (where he was nurs'd) 9 yre of her at Mrs. Judith Cowfield at Lappiton / his nurse says he is 41 years old 3 days before Michaelmas last according to Catherine Bowen his nurse to ye best of her memory'.

A manuscript containing works of Dafydd ap Gwilym 'yr Ofydd Cymreig. A gasclwyd allan o amryw Lyfrau gan Richd. Thomas A.B. e Coll. Jes. Oxon. 1778'. The collection contains eighty-one pieces.

A manuscript containing 'Lexicon Cambro-Britannicum' by William Gambold, late of Exeter College, Oxford, later rector of Puncheston in Pembrokeshire. Part i of the manuscript contains an English-Welsh dictionary of '88 sheets, writ in 7 months' and completed 'Sep. 14. 1722'. The material was 'collected out of Dr. Davies's Latin-Welsh Dictionary, the Welsh translation of the holy Bible, several approved Welsh Authors, and common use'. There are three columns to each folio. Part ii contains a Welsh-English dictionary of '36 sheets', begun 'Nov. 27. 1721' and completed 'Feby. 17th 1721/2'. There are three columns to each folio.

A manuscript containing poetry by Bedo Brwynllys, Dafydd ab Edmwnd, Dafydd ap Gwilym and others in the hand of Samuel Williams.

A manuscript in the autograph of Moses Williams entitled 'Proper Names of Men & Women in alphabetical order transcribed out of a MS. at Hengwrt'. The list begins with 'Arawn ab Cynfarch, Brenin yr Alban' and ends with 'Ywerydd M. Cyndelig bannawg g. Earddur ab Mor ab Tegerin'.

Welsh proverbs collected by John Morgan which had been omitted from the Dictionary of Dr John Davies, Mallwyd. Also included in the manuscript are a series of the first couplets of Dafydd ap Gwilym's poems.

A manuscript entitled 'Dyfrif Achwyniad ar y tosdurus Sarrhâd o Ymadrodd Halogedig mewn Cymdeithas'.